Institute of Geochemistry and Petrology, ETH Zurich, Zurich 8092, Switzerland.
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Georgia 30332, USA.
Nature. 2016 Apr 28;532(7600):492-5. doi: 10.1038/nature17401. Epub 2016 Apr 13.
Volcanic eruptions transfer huge amounts of gas to the atmosphere. In particular, the sulfur released during large silicic explosive eruptions can induce global cooling. A fundamental goal in volcanology, therefore, is to assess the potential for eruption of the large volumes of crystal-poor, silicic magma that are stored at shallow depths in the crust, and to obtain theoretical bounds for the amount of volatiles that can be released during these eruptions. It is puzzling that highly evolved, crystal-poor silicic magmas are more likely to generate volcanic rocks than plutonic rocks. This observation suggests that such magmas are more prone to erupting than are their crystal-rich counterparts. Moreover, well studied examples of largely crystal-poor eruptions (for example, Katmai, Taupo and Minoan) often exhibit a release of sulfur that is 10 to 20 times higher than the amount of sulfur estimated to be stored in the melt. Here we argue that these two observations rest on how the magmatic volatile phase (MVP) behaves as it rises buoyantly in zoned magma reservoirs. By investigating the fluid dynamics that controls the transport of the MVP in crystal-rich and crystal-poor magmas, we show how the interplay between capillary stresses and the viscosity contrast between the MVP and the host melt results in a counterintuitive dynamics, whereby the MVP tends to migrate efficiently in crystal-rich parts of a magma reservoir and accumulate in crystal-poor regions. The accumulation of low-density bubbles of MVP in crystal-poor magmas has implications for the eruptive potential of such magmas, and is the likely source of the excess sulfur released during explosive eruptions.
火山喷发将大量气体输送到大气中。特别是,在大型硅质爆发性喷发过程中释放的硫会导致全球降温。因此,火山学的一个基本目标是评估储存在地壳浅层的大量低结晶硅质岩浆喷发的潜力,并为这些喷发过程中可能释放的挥发物量获得理论限制。令人费解的是,高度演化、低结晶硅质岩浆比深成岩石更有可能产生火山岩。这一观察结果表明,与富含晶体的同类物质相比,这种岩浆更容易喷发。此外,经过充分研究的大量低结晶喷发实例(例如卡特迈、陶波和米诺安)通常表现出的硫释放量比估计储存在熔体中的硫量高出 10 到 20 倍。在这里,我们认为这两个观察结果取决于岩浆挥发性相 (MVP) 在分带岩浆储层中浮力上升时的行为方式。通过研究控制富含晶体和低结晶岩浆中 MVP 传输的流体动力学,我们展示了毛细应力和 MVP 与主熔体之间的粘度对比之间的相互作用如何导致反直觉的动力学,即 MVP 倾向于在岩浆储层的富含晶体部分高效迁移并在低结晶区域积累。低密度 MVP 气泡在低结晶岩浆中的积累对这种岩浆的喷发潜力有影响,也是爆发性喷发中释放过量硫的可能来源。