Department of Physics, University of California at Berkeley, Berkeley, California 94720, USA.
Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
Nat Mater. 2016 Aug;15(8):840-4. doi: 10.1038/nmat4653. Epub 2016 May 30.
Layer-stacking domain walls in bilayer graphene are emerging as a fascinating one-dimensional system that features stacking solitons structurally and quantum valley Hall boundary states electronically. The interactions between electrons in the 2D graphene domains and the one-dimensional domain-wall solitons can lead to further new quantum phenomena. Domain-wall solitons of varied local structures exist along different crystallographic orientations, which can exhibit distinct electrical, mechanical and optical properties. Here we report soliton-dependent 2D graphene plasmon reflection at different 1D domain-wall solitons in bilayer graphene using near-field infrared nanoscopy. We observe various domain-wall structures in mechanically exfoliated graphene bilayers, including network-forming triangular lattices, individual straight or bent lines, and even closed circles. The near-field infrared contrast of domain-wall solitons arises from plasmon reflection at domain walls, and exhibits markedly different behaviours at the tensile- and shear-type domain-wall solitons. In addition, the plasmon reflection at domain walls exhibits a peculiar dependence on electrostatic gating. Our study demonstrates the unusual and tunable coupling between 2D graphene plasmons and domain-wall solitons.
双层石墨烯中的层状畴壁作为一种迷人的一维体系正在出现,其结构上具有堆积孤子,电子上具有量子谷霍尔边界态。二维石墨烯畴中的电子与一维畴壁孤子之间的相互作用可能导致进一步的新量子现象。具有不同局部结构的畴壁孤子沿着不同的晶体取向存在,可表现出不同的电学、力学和光学性质。在这里,我们使用近场红外纳米显微镜报告了双层石墨烯中不同一维畴壁孤子上依赖于孤子的二维石墨烯等离子体反射。我们观察到机械剥离的双层石墨烯中的各种畴壁结构,包括形成网络的三角形晶格、单个的直线或弯曲线,甚至封闭的圆。畴壁孤子的近场红外对比度源于畴壁处的等离子体反射,并在张型和剪型畴壁孤子处表现出明显不同的行为。此外,等离子体在畴壁处的反射表现出对静电门控的特殊依赖性。我们的研究证明了二维石墨烯等离子体和畴壁孤子之间的不寻常和可调谐的耦合。