Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of Sciences , Beijing 100083, China.
School of Materials Science and Engineering, Georgia Institute of Technology , Atlanta, Georgia 30332-0245, United States.
ACS Nano. 2016 Dec 27;10(12):11420-11427. doi: 10.1021/acsnano.6b06998. Epub 2016 Dec 8.
With a promising prospect of light-emitting diodes as an attractive alternative to conventional light sources, remaining challenges still cannot be addressed owing to their limited efficiency. Among the continued scientific efforts, significant improvement on the emission efficiency has been achieved via either piezo-phototronic effect-based strain modulation or resonant excitation of plasmons in metallic nanostructures. Here, we present the investigation on the coupling process between piezo-phototronic effect and localized surface plasmonic resonance for enhancing the photoluminescence of InGaN/GaN quantum wells coated with Ag nanoparticles. The underlying physical mechanism of experimental results originates from tuning plasmonic resonance controlled by the shift of emission wavelength via piezo-phototronic effect, and it is further confirmed with the support of theoretical calculations. As a result, our research provides an approach to the integration of plasmonics with piezo-phototronic effect and brings widespread applications to high-efficiency artificial lighting, on-chip integrated plasmonic circuits, subwavelength optical communication, and micro-optoelectronic mechanical systems.
由于发光二极管作为传统光源的一种有吸引力的替代品,其效率有限,仍然存在一些尚未解决的挑战。在持续的科学努力中,通过基于压电 - 光致电子效应的应变调制或在金属纳米结构中共振激发等离子体,在发射效率方面取得了重大进展。在这里,我们研究了压电 - 光致电子效应和局域表面等离激元共振之间的耦合过程,以增强涂覆有银纳米颗粒的 InGaN/GaN 量子阱的光致发光。实验结果的潜在物理机制源于通过压电 - 光致电子效应调谐等离子体共振来控制发射波长的位移,并且通过理论计算得到了进一步证实。因此,我们的研究为将等离子体学与压电 - 光致电子效应相结合提供了一种方法,并为高效人工照明、片上集成等离子体电路、亚波长光通信和微光机电系统带来了广泛的应用。