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2014 - 2015年北京主要空气污染物特征分析

Characterization of criteria air pollutants in Beijing during 2014-2015.

作者信息

Guo Hao, Wang Yungang, Zhang Hongliang

机构信息

Department of Civil and Environmental Engineering, Louisiana State University, Baton Rouge, LA 70803, USA.

GAGO Inc., San Jose, CA 95035, USA.

出版信息

Environ Res. 2017 Apr;154:334-344. doi: 10.1016/j.envres.2017.01.029. Epub 2017 Feb 1.

Abstract

One year-long criteria air pollutants data collected in Beijing were analyzed in this paper, which can support the research on formation, transport and human health effects of air pollutants. This is the first time to study the spatial and temporal variations of criteria pollutants in Beijing using hourly observational data from 12 sites between June 2014 and May 2015 released by the Ministry of Environmental Protection (MEP) of China. Beijing is facing tremendous air pollution as the daily averaged PM (particulate matter with aerodynamic diameter less than 2.5µm) concentrations in all sites exceeding the Chinese Ambient Air Quality Standards (CAAQS) Grade I & II standards (15 and 35µg/m). Slightly differences in PM and ozone (O) were observed between sites at the urban and rural areas. Pearson correlation coefficients show that most pollutants are temporally correlated in Beijing except for O. The coefficients of divergence (COD) indicate that PM is associated at most sites with only one rural site (Dingling) having observable difference and one site may be insufficient for monitoring surrounding area. The 8h peak O (O-8h) also correlates at different sites but with one urban site (Haidianquwanliu) different from others. In addition, an extreme PM event (hourly average concentration exceeding 300μg/m for ~40h) was examined with the consideration of meteorological conditions. Southerly wind with low speed and high relative humidity allow the accumulation of pollutants while northerly wind with high speed and low relative humidity result in good air quality.

摘要

本文分析了在北京收集的为期一年的环境空气质量标准污染物数据,这些数据可支持对空气污染物的形成、传输及对人体健康影响的研究。这是首次利用中国环境保护部(MEP)发布的2014年6月至2015年5月期间12个站点的小时观测数据,研究北京环境空气质量标准污染物的时空变化。北京正面临着严重的空气污染问题,所有站点的日均PM(空气动力学直径小于2.5μm的颗粒物)浓度均超过中国环境空气质量标准(CAAQS)的一级和二级标准(15和35μg/m³)。城乡站点之间的PM和臭氧(O₃)略有差异。Pearson相关系数表明,除O₃外,北京的大多数污染物在时间上具有相关性。离散系数(COD)表明,大多数站点的PM与仅一个农村站点(定陵)存在明显差异,一个站点可能不足以监测周边地区。不同站点的8小时峰值O₃(O₃-8h)也具有相关性,但有一个城市站点(海淀区万柳)与其他站点不同。此外,还考虑了气象条件,对一次极端PM事件(小时平均浓度超过300μg/m³约40小时)进行了研究。低速和高相对湿度的南风会导致污染物积聚,而高速和低相对湿度的北风则会带来良好的空气质量。

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