Mankowsky R, Liu B, Rajasekaran S, Liu H Y, Mou D, Zhou X J, Merlin R, Först M, Cavalleri A
Max Planck Institute for the Structure and Dynamics of Matter, 22761 Hamburg, Germany.
University of Hamburg, 22761 Hamburg, Germany.
Phys Rev Lett. 2017 Mar 17;118(11):116402. doi: 10.1103/PhysRevLett.118.116402. Epub 2017 Mar 15.
We study the response of the one-dimensional charge density wave in K_{0.3}MoO_{3} to different types of excitation with femtosecond optical pulses. We compare direct excitation of the lattice at midinfrared frequencies with injection of quasiparticles across the low energy charge density wave gap and with charge transfer excitation in the near infrared. For all three cases, we observe a fluence threshold above which the amplitude-mode oscillation frequency is softened and the mode becomes increasingly damped. We show that all the data can be collapsed onto a universal curve in which the melting of the charge density wave occurs abruptly at a critical lattice excursion. These data highlight the existence of a universal stability limit for a charge density wave, reminiscent of the Lindemann criterion for the melting of a crystal lattice.
我们研究了K₀.₃MoO₃中一维电荷密度波对不同类型飞秒光脉冲激发的响应。我们将中红外频率下晶格的直接激发与跨越低能电荷密度波能隙的准粒子注入以及近红外中的电荷转移激发进行了比较。对于所有这三种情况,我们都观察到一个通量阈值,高于该阈值时,振幅模式振荡频率会变软,且模式的阻尼越来越大。我们表明,所有数据都可以合并到一条通用曲线上,在该曲线上电荷密度波在临界晶格偏移时突然熔化。这些数据突出了电荷密度波存在一个通用的稳定性极限,这让人想起晶格熔化的林德曼判据。