Rudolf Peierls Centre for Theoretical Physics, University of Oxford, Oxford OX1 3NP, UK.
Chem Soc Rev. 2017 Sep 18;46(18):5508-5518. doi: 10.1039/c7cs00087a.
Designing microscopic and nanoscopic self-propelled particles and characterising their motion have become a major scientific challenge over the past few decades. To this purpose, phoretic effects, namely propulsion mechanisms relying on local field gradients, have been the focus of many theoretical and experimental studies. In this review, we adopt a tutorial approach to present the basic physical mechanisms at stake in phoretic motion, and describe the different experimental works that led to the fabrication of active particles based on this principle. We also present the collective effects observed in assemblies of interacting active colloids, and the theoretical tools that have been used to describe phoretic and hydrodynamic interactions.
在过去的几十年中,设计微观和纳米自推进粒子并对其运动进行描述已成为一个重大的科学挑战。为此,趋磁效应(即依赖于局部场梯度的推进机制)一直是许多理论和实验研究的重点。在这篇综述中,我们采用教程的方法介绍了趋磁运动中涉及的基本物理机制,并描述了基于该原理制造活性粒子的不同实验工作。我们还介绍了相互作用的活性胶体组装体中观察到的集体效应,以及用于描述趋磁和水动力相互作用的理论工具。