Langer F, Hohenleutner M, Huttner U, Koch S W, Kira M, Huber R
Department of Physics, University of Regensburg, 93040 Regensburg, Germany.
Department of Physics, University of Marburg, 35032 Marburg, Germany.
Nat Photonics. 2017 Apr;11(4):227-231. doi: 10.1038/nphoton.2017.29. Epub 2017 Mar 13.
High-harmonic (HH) generation in crystalline solids1-6 marks an exciting development, with potential applications in high-efficiency attosecond sources7, all-optical bandstructure reconstruction8,9, and quasiparticle collisions10,11. Although the spectral1-4 and temporal shape5 of the HH intensity has been described microscopically1-6,12, the properties of the underlying HH carrier wave have remained elusive. Here we analyse the train of HH waveforms generated in a crystalline solid by consecutive half cycles of the same driving pulse. Extending the concept of frequency combs13-15 to optical clock rates, we show how the polarization and carrier-envelope phase (CEP) of HH pulses can be controlled by crystal symmetry. For some crystal directions, we can separate two orthogonally polarized HH combs mutually offset by the driving frequency to form a comb of even and odd harmonic orders. The corresponding CEP of successive pulses is constant or offset by π, depending on the polarization. In the context of a quantum description of solids, we identify novel capabilities for polarization- and phase-shaping of HH waveforms that cannot be accessed with gaseous sources.
晶体固体中的高谐波(HH)产生1-6标志着一项令人兴奋的进展,在高效阿秒光源7、全光能带结构重构8,9以及准粒子碰撞10,11等方面具有潜在应用。尽管已经从微观角度1-6,12描述了HH强度的光谱1-4和时间形状5,但潜在的HH载波的特性仍然难以捉摸。在这里,我们分析了由同一驱动脉冲的连续半周期在晶体固体中产生的HH波形序列。将频率梳13-15的概念扩展到光学时钟速率,我们展示了如何通过晶体对称性来控制HH脉冲的偏振和载波包络相位(CEP)。对于某些晶体方向,我们可以分离出两个相互正交偏振的HH梳,它们相互偏移驱动频率,从而形成一个偶次和奇次谐波阶数的梳。连续脉冲的相应CEP是恒定的,或者根据偏振偏移π。在固体的量子描述背景下,我们确定了HH波形偏振和相位整形的新能力,这是气态源无法实现的。