Leyden Matthew R, Meng Lingqiang, Jiang Yan, Ono Luis K, Qiu Longbin, Juarez-Perez Emilio J, Qin Chuanjiang, Adachi Chihaya, Qi Yabing
Energy Materials and Surface Sciences Unit (EMSS), Okinawa Institute of Science and Technology Graduate University (OIST) , 1919-1 Tancha, Onna-son, Kunigami-gun, Okinawa 904-0495, Japan.
Center for Organic Photonics and Electronics Research (OPERA), Kyushu University , 744 Motooka, Nishi-ku, Fukuoka 819-0395, Japan.
J Phys Chem Lett. 2017 Jul 20;8(14):3193-3198. doi: 10.1021/acs.jpclett.7b01093. Epub 2017 Jun 29.
Organo-lead-halide perovskites are promising materials for optoelectronic applications. Perovskite solar cells have reached power conversion efficiencies of over 22%, and perovskite light-emitting diodes have recently achieved over 11% external quantum efficiency. To date, most research on perovskite light-emitting diodes has focused on solution-processed films. There are many advantages of a vapor-based growth process to prepare perovskites, including ease of patterning, ability to batch process, and material compatibility. We investigated an all-vapor perovskite growth process by chemical vapor deposition and demonstrated luminance up to 560 cd/m.
有机铅卤化物钙钛矿是用于光电子应用的有前途的材料。钙钛矿太阳能电池的功率转换效率已超过22%,并且钙钛矿发光二极管最近已实现超过11%的外量子效率。迄今为止,大多数关于钙钛矿发光二极管的研究都集中在溶液处理的薄膜上。基于气相的钙钛矿生长工艺有许多优点,包括易于图案化、批量处理能力和材料兼容性。我们通过化学气相沉积研究了全气相钙钛矿生长工艺,并证明了高达560 cd/m的亮度。