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阿海珐集团(法国)拉阿格后处理厂影响下的大气氚浓度及本底水平。

Atmospheric tritium concentrations under influence of AREVA NC La Hague reprocessing plant (France) and background levels.

作者信息

Connan O, Hébert D, Solier L, Maro D, Pellerin G, Voiseux C, Lamotte M, Laguionie P

机构信息

Institut de Radioprotection et de Sûreté Nucléaire (IRSN), PRP-ENV/SERIS/LRC, Radioecology Laboratory, BP10, Rue Max Pol Fouchet, 50130 Cherbourg-Octeville, France.

Institut de Radioprotection et de Sûreté Nucléaire (IRSN), PRP-ENV/SERIS/LRC, Radioecology Laboratory, BP10, Rue Max Pol Fouchet, 50130 Cherbourg-Octeville, France.

出版信息

J Environ Radioact. 2017 Oct;177:184-193. doi: 10.1016/j.jenvrad.2017.06.015. Epub 2017 Jul 6.

Abstract

In-air tritium measurements were conducted around the AREVA NC La Hague reprocessing plant, as well as on other sites that are not impacted by the nuclear industry in northwest of France. The results indicate that the dominant tritium form around the AREVA site is HT (86%). HT and HTO levels are lower than 5 and 1 Bq. m for hourly samples taken in the plume. No tritiated organic molecules (TOM) were detected. 26 measurement campaigns were performed and links were established between near-field Kr, HT and HTO activities. Environmental measurements are in line with those taken at the discharge stack, and tend to demonstrate that there are no rapid changes in the tritium forms released. Out of the influence of any nuclear activities, the levels measured were below 13 mBq.m for HT and 5 mBq.m for HTO (<0.5 Bq. L). HTO level in air seems to be influenced by HTO activities in surrounding seawater.

摘要

在阿海珐集团(AREVA)NC拉阿格后处理厂周围以及法国西北部其他未受核工业影响的地点进行了空气中氚的测量。结果表明,阿海珐集团厂区周围氚的主要形态是HT(86%)。对于在羽流中采集的每小时样本,HT和HTO水平分别低于5 Bq/m³和1 Bq/m³。未检测到含氚有机分子(TOM)。开展了26次测量活动,并建立了近场氪、HT和HTO活度之间的联系。环境测量结果与排放烟囱处的测量结果一致,且倾向于表明所释放的氚形态没有快速变化。在不受任何核活动影响的区域,所测HT水平低于13 mBq/m³,HTO水平低于5 mBq/m³(<0.5 Bq/L)。空气中的HTO水平似乎受到周围海水中HTO活度的影响。

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