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碳纳米管中的相干等离子体与声子-等离子体共振

Coherent Plasmon and Phonon-Plasmon Resonances in Carbon Nanotubes.

作者信息

Falk Abram L, Chiu Kuan-Chang, Farmer Damon B, Cao Qing, Tersoff Jerry, Lee Yi-Hsien, Avouris Phaedon, Han Shu-Jen

机构信息

IBM T. J. Watson Research Center, Yorktown Heights, New York 10598, USA.

Department of Materials Science and Engineering, National Tsing-Hua University, Hsinchu, Taiwan 30013.

出版信息

Phys Rev Lett. 2017 Jun 23;118(25):257401. doi: 10.1103/PhysRevLett.118.257401. Epub 2017 Jun 22.

Abstract

Carbon nanotubes provide a rare access point into the plasmon physics of one-dimensional electronic systems. By assembling purified nanotubes into uniformly sized arrays, we show that they support coherent plasmon resonances, that these plasmons couple to nanotube and substrate phonons, and that the resulting phonon-plasmon resonances have quality factors as high as 10. Because nanotube plasmons intensely strengthen electromagnetic fields and light-matter interactions, they provide a compelling platform for surface-enhanced spectroscopy and tunable optical devices at deep-subwavelength scales.

摘要

碳纳米管为研究一维电子系统的等离激元物理提供了一个难得的切入点。通过将纯化后的纳米管组装成尺寸均匀的阵列,我们发现它们支持相干等离激元共振,这些等离激元与纳米管和基底声子耦合,并且由此产生的声子 - 等离激元共振的品质因数高达10。由于纳米管等离激元能强烈增强电磁场和光与物质的相互作用,它们为深亚波长尺度下的表面增强光谱学和可调谐光学器件提供了一个极具吸引力的平台。

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