Zhou Hengjie, Su Shaojian, Qiu Weibin, Zhao Zeyang, Lin Zhili, Qiu Pingping, Kan Qiang
Fujian Key Laboratory of Light Propagation and Transformation, College of Information, Science and Engineering, Huaqiao University, Xiamen 361021, China.
Fujian Key Laboratory of Semiconductor Materials and Applications, Xiamen University, Xiamen 361005, China.
Nanomaterials (Basel). 2020 Jan 29;10(2):236. doi: 10.3390/nano10020236.
Multiple Fano resonances (FRs) can be produced by destroying the symmetry of structure or adding additional nanoparticles without changing the spatial symmetry, which has been proved in noble metal structures. However, due to the disadvantages of low modulation depth, large damping rate, and broadband spectral responses, many resonance applications are limited. In this research paper, we propose a graphene plasmonic metamolecule (PMM) by adding an additional 12 nanodiscs around a graphene heptamer, where two Fano resonance modes with different wavelengths are observed in the extinction spectrum. The competition between the two FRs as well as the modulation depth of each FR is investigated by varying the materials and the geometrical parameters of the nanostructure. A simple trimer model, which emulates the radical distribution of the PMM, is employed to understand the electromagnetic field behaviors during the variation of the parameters. Our proposed graphene nanostructures might find significant applications in the fields of single molecule detection, chemical or biochemical sensing, and nanoantenna.
通过破坏结构的对称性或添加额外的纳米粒子而不改变空间对称性,可以产生多个法诺共振(FRs),这已在贵金属结构中得到证实。然而,由于调制深度低、阻尼率大以及宽带光谱响应等缺点,许多共振应用受到限制。在本研究论文中,我们通过在石墨烯七聚体周围添加额外的12个纳米盘提出了一种石墨烯等离子体超分子(PMM),在消光光谱中观察到了两种不同波长的法诺共振模式。通过改变纳米结构的材料和几何参数,研究了两种FRs之间的竞争以及每个FR的调制深度。采用一个简单的三聚体模型来模拟PMM的基团分布,以理解参数变化过程中的电磁场行为。我们提出的石墨烯纳米结构可能在单分子检测、化学或生化传感以及纳米天线等领域找到重要应用。