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用于传感应用的偏振不变等离子体激元纳米结构。

Polarization invariant plasmonic nanostructures for sensing applications.

机构信息

Nanophotonics Lab, School of EEE, OPTIMUS, Nanyang Technological University, 50 Nanyang Avenue, Singapore, 639798, Singapore.

Institute of Material Research and Engineering, Agency of Science, Technology (A*Star), 3 Research Link, Singapore, 117602, Singapore.

出版信息

Sci Rep. 2017 Aug 8;7(1):7539. doi: 10.1038/s41598-017-08020-y.

Abstract

Optics-based sensing platform working under unpolarized light illumination is of practical importance in the sensing applications. For this reason, sensing platforms based on localized surface plasmons are preferred to their integrated optics counterparts for their simple mode excitation and inexpensive implementation. However, their optical response under unpolarized light excitation is typically weak due to their strong polarization dependence. Herein, the role of rotational symmetry for realizing robust sensing platform exhibiting strong optical contrast and high sensitivity is explored. Specifically, gammadion and star-shaped gold nanostructures with different internal and external rotational symmetries are fabricated and studied in detail, from which their mode characteristics are demonstrated as superposition of their constituent longitudinal plasmons that are in conductive coupling with each other. We demonstrate that introducing and increasing internal rotational symmetry would lead to the enhancement in optical contrast up to ~3x under unpolarized light illumination. Finally, we compare the sensing performances of rotationally symmetric gold nanostructures with a more rigorous figure-of-merit based on sensitivity, Q-factor, and spectral contrast.

摘要

基于光学的传感平台在非偏振光照明下工作在传感应用中具有实际意义。出于这个原因,基于局域表面等离子体的传感平台因其简单的模式激发和廉价的实现而优于其集成光学对应物。然而,由于它们强烈的偏振依赖性,它们在非偏振光激发下的光学响应通常较弱。在本文中,探索了旋转对称在实现具有强光学对比度和高灵敏度的稳健传感平台中的作用。具体来说,制造并详细研究了具有不同内部和外部旋转对称性的伽马形和星形金纳米结构,从中展示了它们的模式特征,即它们的组成纵向等离子体的叠加,这些等离子体彼此之间具有导电性耦合。我们证明,引入和增加内部旋转对称性将导致光学对比度在非偏振光照射下提高约 3 倍。最后,我们比较了具有更严格的基于灵敏度、Q 因子和光谱对比度的品质因数的旋转对称金纳米结构的传感性能。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6596/5548906/3256c791bd47/41598_2017_8020_Fig1_HTML.jpg

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