Department of Applied Physics , The Hong Kong Polytechnic University , Hong Kong.
ACS Appl Mater Interfaces. 2018 Aug 8;10(31):25834-25840. doi: 10.1021/acsami.7b07668. Epub 2017 Aug 28.
Organic electrochemical transistors (OECTs) have been successfully employed for a variety of applications , especially chemical and biological sensing. Although the device response to analytes can be directly monitored by measuring steady-state channel currents of the devices, it is challenging to obtain stable signals with high signal-to-noise ratios. In this work, we developed a novel method for electrochemical sensing by measuring both the transconductance and the phase of the AC channel current for the first time. Then we successfully realized highly sensitive ion strength sensors and dopamine sensors based on the AC method. Our results indicate that the AC method is more sensitive than typical DC methods and can provide more stable data in sensing applications. Considering that the sensors can be conveniently integrated with AC circuits, this technology is expected to find broad applications in the future.
有机电化学晶体管 (OECT) 已成功应用于各种领域,尤其是化学和生物传感。尽管可以通过测量器件的稳态沟道电流来直接监测器件对分析物的响应,但获得具有高信噪比的稳定信号具有挑战性。在这项工作中,我们首次开发了一种通过同时测量交流沟道电流的跨导和相位来进行电化学传感的新方法。然后,我们成功地基于交流方法实现了高灵敏度的离子强度传感器和多巴胺传感器。我们的结果表明,交流方法比典型的直流方法更灵敏,并且在传感应用中可以提供更稳定的数据。鉴于传感器可以与交流电路方便地集成,这项技术有望在未来得到广泛应用。