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通过跟踪电偶极子和磁偶极子模式的相互作用来分析本征等离子体手性。

Analyzing intrinsic plasmonic chirality by tracking the interplay of electric and magnetic dipole modes.

机构信息

Chongqing Engineering Laboratory for Detection, Control and Integrated System, School of Computer Science and Information Engineering, Chongqing Technology and Business University, Chongqing, 400067, P. R. China.

Soft Matter and Interdisciplinary Research Center, College of Physics, Chongqing University, Chongqing, 400044, P. R. China.

出版信息

Sci Rep. 2017 Sep 11;7(1):11151. doi: 10.1038/s41598-017-11571-9.

DOI:10.1038/s41598-017-11571-9
PMID:28894208
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC5593961/
Abstract

Plasmonic chirality represents significant potential for novel nanooptical devices due to its association with strong chiroptical responses. Previous reports on plasmonic chirality mechanism mainly focus on phase retardation and coupling. In this paper, we propose a model similar to the chiral molecules for explaining the intrinsic plasmonic chirality mechanism of varies 3D chiral structures quantitatively based on the interplay and mixing of electric and magnetic dipole modes (directly from electromagnetic field numerical simulations), which forms mixed electric and magnetic polarizability.

摘要

等离子体手性由于与强手性响应相关联,因此在新型纳米光学器件中有很大的应用潜力。先前关于等离子体手性机制的报告主要集中在相位滞后和耦合上。在本文中,我们提出了一个类似于手性分子的模型,根据电偶极子和磁偶极子模式的相互作用和混合(直接来自电磁场数值模拟)来定量解释各种 3D 手性结构的固有等离子体手性机制,从而形成混合电和磁极化率。

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本文引用的文献

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Tailoring the chirality of light emission with spherical Si-based antennas.用基于 Si 的球形天线调控光发射的手性。
Nanoscale. 2016 May 21;8(19):10441-52. doi: 10.1039/c6nr00676k. Epub 2016 May 4.
2
Quantitatively analyzing the mechanism of giant circular dichroism in extrinsic plasmonic chiral nanostructures by tracking the interplay of electric and magnetic dipoles.通过追踪电偶极子和磁偶极子的相互作用来定量分析外在等离子体手性纳米结构中巨圆二色性的机制。
Nanoscale. 2016 Feb 14;8(6):3720-8. doi: 10.1039/c5nr08527f. Epub 2016 Jan 27.
3
Tailoring chiro-optical effects by helical nanowire arrangement.
电磁手性:从基础到非传统手性光学现象
Light Sci Appl. 2020 Sep 2;9:139. doi: 10.1038/s41377-020-00367-8. eCollection 2020.
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Spin-preserving chiral photonic crystal mirror.自旋保持手性光子晶体镜
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5
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Sensors (Basel). 2020 Feb 10;20(3):944. doi: 10.3390/s20030944.
通过螺旋纳米线排列定制手性光学效应。
Nanoscale. 2015 Nov 21;7(43):18081-8. doi: 10.1039/c5nr04674b.
4
Triple-helical nanowires by tomographic rotatory growth for chiral photonics.用于手性光子学的断层旋转生长三螺旋纳米线。
Nat Commun. 2015 Mar 18;6:6484. doi: 10.1038/ncomms7484.
5
Plasmonic DNA-origami nanoantennas for surface-enhanced Raman spectroscopy.等离子体 DNA 折纸纳米天线用于表面增强拉曼光谱。
Nano Lett. 2014 May 14;14(5):2914-9. doi: 10.1021/nl5009635. Epub 2014 Apr 25.
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Chiral plasmonic DNA nanostructures with switchable circular dichroism.手性等离子体 DNA 纳米结构具有可切换的圆二色性。
Nat Commun. 2013;4:2948. doi: 10.1038/ncomms3948.
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Interpreting chiral nanophotonic spectra: the plasmonic Born-Kuhn model.解析手性纳米光子学光谱:等离子体玻恩-库恩模型。
Nano Lett. 2013;13(12):6238-43. doi: 10.1021/nl403705k. Epub 2013 Nov 27.
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Large-area 3D chiral plasmonic structures.大面积 3D 手性等离子体结构。
ACS Nano. 2013 Jul 23;7(7):6321-9. doi: 10.1021/nn402370x. Epub 2013 Jul 5.
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Chirality and chiroptical effects in plasmonic nanostructures: fundamentals, recent progress, and outlook.手性和手性光学在等离子体纳米结构中的效应:基础、最新进展和展望。
Adv Mater. 2013 May 14;25(18):2517-34. doi: 10.1002/adma.201205178. Epub 2013 Apr 2.
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