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加利福尼亚州部分油气设施的甲烷排放的空气传播测量。

Airborne Methane Emission Measurements for Selected Oil and Gas Facilities Across California.

机构信息

Land Air and Water Resources, University of California , Davis, California 95616, United States.

Scientific Aviation, Inc., Boulder, Colorado 80301, United States.

出版信息

Environ Sci Technol. 2017 Nov 7;51(21):12981-12987. doi: 10.1021/acs.est.7b03254. Epub 2017 Oct 24.

DOI:10.1021/acs.est.7b03254
PMID:29019666
Abstract

We report 65 individual measurements of methane emissions from 24 oil and gas facilities across California. Methane emission rates were estimated using in situ methane and wind velocity measurements from a small aircraft by a novel Gauss' Theorem flux integral approach. The estimates are compared with annual mean emissions reported to the U.S. Environmental Protection Agency (USEPA) and the California Air Resources Board (CARB) through their respective greenhouse gas reporting programs. The average emissions from 36 measurements of 10 gas storage facilities were within a factor of 2 of emissions reported to USEPA or CARB, though large variance was observed and the reporting database did not contain all of the facilities. In contrast, average emissions from 15 measurements of the three refineries were roughly an order of magnitude more than reported to the USEPA or CARB. The remaining measurements suggest compressor emissions are variable and perhaps slightly larger than reported, and emissions from one oil production facility were roughly concordant with a separate (not GHG reporting) bottom-up estimate from other work. Together, these results provide an initial facility-specific survey of methane emissions from California oil and natural gas infrastructure with observed variability suggesting the need for expanded measurements in the future.

摘要

我们报告了来自加利福尼亚州 24 个石油和天然气设施的 65 项甲烷排放的单独测量值。甲烷排放率是使用小型飞机上的原位甲烷和风速测量值,通过一种新的高斯定理通量积分方法来估算的。这些估计值与通过各自的温室气体报告计划向美国环境保护署(USEPA)和加利福尼亚州空气资源委员会(CARB)报告的年平均值进行了比较。通过 10 个天然气储存设施的 36 次测量得出的平均排放量与向 USEPA 或 CARB 报告的排放量相差 2 倍以内,尽管观察到了很大的差异,而且报告数据库并未包含所有设施。相比之下,从三个炼油厂的 15 次测量得出的平均排放量比向 USEPA 或 CARB 报告的排放量大约高出一个数量级。其余的测量结果表明,压缩机排放量是可变的,而且可能略高于报告的排放量,而一个石油生产设施的排放量与其他工作的另一个(非温室气体报告)自下而上的估算大致相符。总的来说,这些结果提供了对加利福尼亚州石油和天然气基础设施甲烷排放的初步设施特定调查,观察到的可变性表明未来需要进行更多的测量。

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