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硅发光二极管中的室温磁光效应。

Room temperature magneto-optic effect in silicon light-emitting diodes.

作者信息

Chiodi F, Bayliss S L, Barast L, Débarre D, Bouchiat H, Friend R H, Chepelianskii A D

机构信息

Centre de Nanosciences et de Nanotechnologies, CNRS, Univ. Paris-Sud, Université Paris-Saclay, C2N-Orsay, Orsay, 91405, France.

Laboratoire de Physique des solides, CNRS, Univ. Paris-Sud, Université Paris-Saclay, LPS-Orsay, Orsay, 91405, France.

出版信息

Nat Commun. 2018 Jan 26;9(1):398. doi: 10.1038/s41467-017-02804-6.

Abstract

In weakly spin-orbit coupled materials, the spin-selective nature of recombination can give rise to large magnetic-field effects, e.g. on the electro-luminescence of molecular semiconductors. Although silicon has weak spin-orbit coupling, observing spin-dependent recombination through magneto-electroluminescence is challenging: silicon's indirect band-gap causes an inefficient emission and it is difficult to separate spin-dependent phenomena from classical magneto-resistance effects. Here we overcome these challenges and measure magneto-electroluminescence in silicon light-emitting diodes fabricated via gas immersion laser doping. These devices allow us to achieve efficient emission while retaining a well-defined geometry, thus suppressing classical magnetoresistance effects to a few percent. We find that electroluminescence can be enhanced by up to 300% near room temperature in a seven Tesla magnetic field, showing that the control of the spin degree of freedom can have a strong impact on the efficiency of silicon LEDs.

摘要

在弱自旋轨道耦合材料中,复合过程的自旋选择性会产生显著的磁场效应,例如对分子半导体的电致发光的影响。尽管硅具有较弱的自旋轨道耦合,但通过磁电致发光观测自旋相关的复合过程具有挑战性:硅的间接带隙导致发光效率低下,并且难以将自旋相关现象与经典磁阻效应区分开来。在此,我们克服了这些挑战,测量了通过气体浸没激光掺杂制造的硅发光二极管中的磁电致发光。这些器件使我们能够在保持明确几何形状的同时实现高效发光,从而将经典磁阻效应抑制到百分之几。我们发现,在七特斯拉磁场中,接近室温时电致发光可增强高达300%,这表明对自旋自由度的控制会对硅发光二极管的效率产生强烈影响。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/855c/5785965/c5a5d2200e60/41467_2017_2804_Fig1_HTML.jpg

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