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巴西环境介质中新兴关注污染物的发生、控制和归宿。

Occurrence, control and fate of contaminants of emerging concern in environmental compartments in Brazil.

机构信息

Department of Sanitary and Environmental Engineering, Research Group on Environmental Applications of Advanced Oxidation Processes, Universidade Federal de Minas Gerais. Av.Antônio Carlos, 6627, Belo Horizonte - MG, Brazil, 31270-901.

Department of Sanitary and Environmental Engineering, Research Group on Environmental Applications of Advanced Oxidation Processes, Universidade Federal de Minas Gerais. Av.Antônio Carlos, 6627, Belo Horizonte - MG, Brazil, 31270-901.

出版信息

J Hazard Mater. 2019 Jun 15;372:17-36. doi: 10.1016/j.jhazmat.2018.04.043. Epub 2018 Apr 22.

Abstract

This is the first review to present data obtained in Brazil over the years regarding contaminants of emerging concern (CEC) and to contrast it with contamination in other countries. Data gathered indicated that caffeine, paracetamol, atenolol, ibuprofen, cephalexin and bisphenol A occur in the μg L range in streams near urban areas. While endocrine disruptors are frequently detected in surface waters, highest concentrations account for 17α-ethynylestradiol and 17β-estradiol. Organochlorine pesticides are the most frequently found and persistent in sediments in agricultural regions. Moreover, in tropical agricultural fields, pesticide volatilization and its implications to ecosystem protection must be better investigated. The reality represented here for Brazil may be transposed to other developing countries due to similarities related to primitive basic sanitation infrastructure and economic and social contexts, which contribute to continuous environmental contamination by CEC. Municipal wastewater treatment facilities in Brazil, treat up to the secondary stage and lead to limited CEC removal. This is also true for other nations in Latin America, such as Argentina, Colombia and Mexico. Therefore, it is an urgent priority to improve sanitation infrastructure and, then, the implementation of tertiary treatment shall be imposed.

摘要

这是第一篇综述,呈现了多年来在巴西获得的有关新兴关注污染物(CEC)的数据,并与其他国家的污染情况进行了对比。收集的数据表明,咖啡因、对乙酰氨基酚、阿替洛尔、布洛芬、头孢氨苄和双酚 A 在城市附近溪流中的浓度处于μg/L 范围内。虽然内分泌干扰物经常在地表水中被检测到,但浓度最高的是 17α-乙炔雌二醇和 17β-雌二醇。有机氯农药在农业地区的沉积物中最常被发现且最持久。此外,在热带农业领域,必须更好地研究农药的挥发及其对生态系统保护的影响。由于基本卫生基础设施和经济社会背景相似,巴西的这一现实情况可能会在其他发展中国家出现,这些因素导致 CEC 持续污染环境。巴西的城市废水处理设施仅进行二级处理,导致对 CEC 的去除效果有限。阿根廷、哥伦比亚和墨西哥等拉丁美洲其他国家也是如此。因此,当务之急是改善卫生基础设施,然后强制实施三级处理。

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