Demishev S V, Gilmanov M I, Samarin A N, Semeno A V, Sluchanko N E, Samarin N A, Bogach A V, Shitsevalova N Yu, Filipov V B, Karasev M S, Glushkov V V
Moscow Institute of Physics and Technology, Dolgoprudny, 141700, Moscow region, Russia.
National Research University Higher School of Economics, Moscow, 101000, Russia.
Sci Rep. 2018 May 8;8(1):7125. doi: 10.1038/s41598-018-25464-y.
Introducing of topological insulator concept for fluctuating valence compound - samarium hexaboride - has recently initiated a new round of studies aimed to clarify the nature of the ground state in this extraordinary system with strong electron correlations. Here we discuss the data of magnetic resonance in the pristine single crystals of SmB measured in 60 GHz cavity experiments at temperatures 1.8-300 K. The microwave study as well as the DC resistivity and Hall effect measurements performed for the different states of SmB [110] surface prove definitely the existence of the layer with metallic conductivity increasing under lowering temperature below 5 K. Four lines with the g-factors g ≈ 2 are found to contribute to the ESR-like absorption spectrum that may be attributed to intrinsic paramagnetic centers on the sample's surface, which are robust with respect to the surface treatment. The temperature dependence of integrated intensity I(T) for main paramagnetic signal is found to demonstrate anomalous critical behavior I(T) ~ (T - T) with characteristic temperature T = 5.34 ± 0.05 K and exponent ν = 0.38 ± 0.03 indicating possible magnetic transition at the SmB [110] surface. Additional resonant magnetoabsorption line, which may be associated with either donor-like defects or cyclotron resonance mode corresponding to the mass m ~ 1.2m, is reported.
将拓扑绝缘体概念引入价态波动化合物——六硼化钐,最近引发了新一轮研究,旨在阐明这个具有强电子关联的特殊体系基态的本质。在此,我们讨论在1.8 - 300 K温度下,于60 GHz腔实验中对纯净SmB单晶进行磁共振测量得到的数据。对SmB [110]表面不同状态进行的微波研究以及直流电阻率和霍尔效应测量,明确证实了存在一个金属导电层,其电导率在温度降至5 K以下时增大。发现有四条g因子g≈2的谱线对类似电子自旋共振(ESR)的吸收光谱有贡献,这可能归因于样品表面的本征顺磁中心,这些中心对于表面处理具有稳定性。发现主顺磁信号的积分强度I(T)的温度依赖性表现出反常临界行为I(T) ~ (T - T),特征温度T = 5.34 ± 0.05 K,指数ν = 0.38 ± 0.03,这表明SmB [110]表面可能存在磁转变。还报道了一条额外的共振磁吸收线,它可能与类施主缺陷或对应于有效质量m ~ 1.2m的回旋共振模式有关。