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纳米尺度的光控磁场蚀刻

Optically controlled magnetic-field etching on the nano-scale.

作者信息

Yatsui Takashi, Tsuboi Toshiki, Yamaguchi Maiku, Nobusada Katsuyuki, Tojo Satoshi, Stehlin Fabrice, Soppera Olivier, Bloch Daniel

机构信息

School of Engineering, University of Tokyo, Bunkyo-ku, Tokyo, 113-8656 Japan.

Department of Theoretical and Computational Molecular Science, Institute for Molecular Science, Myodaiji, Okazaki, 444-8585 Japan.

出版信息

Light Sci Appl. 2016 Mar 25;5(3):e16054. doi: 10.1038/lsa.2016.54. eCollection 2016 Mar.

Abstract

Electric and magnetic fields play an important role in both chemical and physical reactions. However, since the coupling efficiency between magnetic fields and electrons is low in comparison with that between electric fields and electrons in the visible wavelength region, the magnetic field is negligible in photo-induced reactions. Here, we performed photo-etching of ZrO nano-stripe structures, and identified an etching-property polarisation dependence. Specifically, the etching rate and etched profiles depend on the structure width. To evaluate this polarisation-dependent etching, we performed numerical calculations using a finite-difference time-domain method. Remarkably, the numerical results revealed that the polarisation-dependent etching properties were determined by the magnetic field distributions, rather than the electric field distributions. As nano-scale structures induce a localised magnetic field, the discovery of this etching dependence on the magnetic field is expected to introduce a new perspective on advanced nano-scale structure fabrication.

摘要

电场和磁场在化学反应和物理反应中都起着重要作用。然而,在可见光波长区域,与电场和电子之间的耦合效率相比,磁场与电子之间的耦合效率较低,因此在光致反应中磁场可忽略不计。在此,我们对ZrO纳米条纹结构进行了光蚀刻,并确定了蚀刻特性的偏振依赖性。具体而言,蚀刻速率和蚀刻轮廓取决于结构宽度。为了评估这种偏振依赖性蚀刻,我们使用时域有限差分法进行了数值计算。值得注意的是,数值结果表明,偏振依赖性蚀刻特性是由磁场分布而非电场分布决定的。由于纳米级结构会产生局部磁场,这种蚀刻对磁场的依赖性的发现有望为先进纳米级结构制造带来新的视角。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9589/6059895/746c48ec8599/lsa201654f1.jpg

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