State Key Laboratory of Surface Physics and Department of Physics , Fudan University , Shanghai 200433 , China.
Collaborative Innovation Center of Advanced Microstructures , Nanjing 210093 , China.
Nano Lett. 2018 Oct 10;18(10):6611-6616. doi: 10.1021/acs.nanolett.8b03267. Epub 2018 Sep 20.
The advent of black phosphorus field-effect transistors (FETs) has brought new possibilities in the study of two-dimensional (2D) electron systems. In a black phosphorus FET, the gate induces highly anisotropic 2D electron and hole gases. Although the 2D hole gas in black phosphorus has reached high carrier mobilities that led to the observation of the integer quantum Hall effect, the improvement in the sample quality of the 2D electron gas (2DEG) has however been only moderate; quantum Hall effect remained elusive. Here, we obtain high quality black phosphorus 2DEG by defining the 2DEG region with a prepatterned graphite local gate. The graphite local gate screens the impurity potential in the 2DEG. More importantly, it electrostatically defines the edge of the 2DEG, which facilitates the formation of well-defined edge channels in the quantum Hall regime. The improvements enable us to observe precisely quantized Hall plateaus in electron-doped black phosphorus FET. Magneto-transport measurements under high magnetic fields further revealed a large effective mass and an enhanced Landé g-factor, which points to strong electron-electron interaction in black phosphorus 2DEG. Such strong interaction may lead to exotic many-body quantum states in the fractional quantum Hall regime.
黑磷场效应晶体管(FET)的出现为二维(2D)电子系统的研究带来了新的可能性。在黑磷 FET 中,栅极诱导出高度各向异性的 2D 电子和空穴气体。尽管黑磷中的 2D 空穴气体已达到很高的载流子迁移率,从而观察到了整数量子霍尔效应,但 2D 电子气体(2DEG)的样品质量的提高却只是适度的;量子霍尔效应仍然难以捉摸。在这里,我们通过使用预先图案化的石墨局部栅极来定义 2DEG 区域,从而获得高质量的黑磷 2DEG。石墨局部栅极屏蔽了 2DEG 中的杂质势。更重要的是,它静电定义了 2DEG 的边缘,这有利于在量子霍尔区形成明确定义的边缘通道。这些改进使我们能够在电子掺杂黑磷 FET 中精确观察到量子化的霍尔平台。在高磁场下的磁输运测量进一步揭示了大的有效质量和增强的朗德 g 因子,这表明在黑磷 2DEG 中存在强烈的电子-电子相互作用。这种强相互作用可能导致分数量子霍尔区中的奇异多体量子态。