Institute of land and urban-rural development, Zhejiang University of Finance & Economics, Hangzhou 310018, PR China.
School of Geographic and Oceanographic Science, Nanjing University, 163 Xianlin Road, Nanjing, Jiangsu, 210023, PR China.
J Hazard Mater. 2019 Feb 15;364:108-116. doi: 10.1016/j.jhazmat.2018.09.094. Epub 2018 Oct 2.
Identifying combined pollution risk areas is difficult because of the complex pollutant sources and heterogeneous soil properties in urban systems. This study used bivariate local Moran's I to analyze the spatial interaction between heavy metals and PAHs, revealed the causes of spatial interaction patterns through PMF, and proposed a risk zoning approach for combined pollution in urban areas. The results showed that both heavy metals and PAHs had high spatial heterogeneity in urban soil. Bivariate LISA maps revealed the spatial interactions between heavy metals and PAHs. The historical area was the hotspot of combined pollution. The overlay of pollutant sources and sinks was responsible for the spatial interaction patterns of combined organic and inorganic pollution. Coal consumption was the main emission source for heavy metal and PAHs pollution, accounting for 31% and 21%, respectively. We used bivariate LISA as the auxiliary variable to reduce the uncertainty of identification combined pollution risk zones. More than 11% of the total area clustered significantly where concentration of both heavy metals and PAHs ware in excess of the risk threshold. This study indicates that we can provide better decision-making support for soil risk management based on the knowledge derived from spatial interaction analysis.
由于城市系统中复杂的污染源和不均匀的土壤特性,识别复合污染区域具有一定的难度。本研究采用双变量局部 Moran's I 分析了重金属和 PAHs 之间的空间相互作用,通过 PMF 揭示了空间相互作用模式的原因,并提出了一种城市地区复合污染的风险分区方法。结果表明,城市土壤中的重金属和 PAHs 均具有较高的空间异质性。双变量 LISA 图谱揭示了重金属和 PAHs 之间的空间相互作用。历史区域是复合污染的热点地区。污染源和汇的叠加是导致有机和无机复合污染空间相互作用模式的原因。煤炭消耗是重金属和 PAHs 污染的主要排放源,分别占 31%和 21%。我们使用双变量 LISA 作为辅助变量,以减少识别复合污染风险区的不确定性。超过 11%的总面积明显聚集,重金属和 PAHs 的浓度均超过风险阈值。本研究表明,我们可以基于空间相互作用分析获得的知识,为土壤风险管理提供更好的决策支持。