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卤化物钙钛矿微腔中的电泵浦极化激子-极化子

Electrically Pumped Polarized Exciton-Polaritons in a Halide Perovskite Microcavity.

作者信息

Wang Tingting, Zang Zhihao, Gao Yuchen, Lyu Chao, Gu Pingfan, Yao Yige, Peng Kai, Watanabe Kenji, Taniguchi Takashi, Liu Xiaoze, Gao Yunan, Bao Wei, Ye Yu

机构信息

State Key Laboratory for Mesoscopic Physics and Frontiers Science Centre for Nano-optoelectronics, School of Physics, Peking University, Beijing 100871, People's Republic of China.

Collaborative Innovation Centre of Quantum Matter, Beijing 100871, People's Republic of China.

出版信息

Nano Lett. 2022 Jul 13;22(13):5175-5181. doi: 10.1021/acs.nanolett.2c00906. Epub 2022 Jun 17.

Abstract

Recently, exciton-polaritons in lead halide perovskite microcavities have been extensively investigated to address striking phenomena such as polariton condensation and quantum emulation. However, a critical step in advancing these findings into practical applications, i.e., realizing electrically pumped perovskite polariton light-emitting devices, has not yet been presented. Here, we devise a new method to combine the device with a microcavity and report the first halide perovskite polariton light-emitting device. Specifically, the device is based on a CsPbBr capacitive structure, which can inject the electrons and holes from the same electrode, conducive to the formation of excitons and simultaneously maintaining the high quality of the microcavity. In addition, highly polarized polariton emissions have been demonstrated due to the optical birefringence in the CsPbBr microplate. This work paves the way for realizing practical polaritonic devices such as high-speed light-emitting devices for information communications and inversionless electrically pumped lasers based on perovskites.

摘要

最近,卤化铅钙钛矿微腔中的激子极化激元已被广泛研究,以探究诸如极化激元凝聚和量子模拟等显著现象。然而,将这些研究成果推进到实际应用中的关键一步,即实现电泵浦钙钛矿极化激元发光器件,尚未达成。在此,我们设计了一种将该器件与微腔相结合的新方法,并报道了首个卤化物钙钛矿极化激元发光器件。具体而言,该器件基于CsPbBr电容结构,其能够从同一电极注入电子和空穴,有利于激子的形成,同时保持微腔的高质量。此外,由于CsPbBr微板中的光学双折射,已证明了高偏振极化激元发射。这项工作为实现诸如用于信息通信的高速发光器件以及基于钙钛矿的无反转电泵浦激光器等实际极化激元器件铺平了道路。

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