Song Han Sung, Lee Gil Ju, Yoo Dong Eun, Kim Yeong Jae, Yoo Young Jin, Lee Dong-Wook, Siva Vantari, Kang Il-Suk, Song Young Min
School of Electrical Engineering and Computer Science, Gwangju Institute of Science and Technology (GIST), 123 Cheomdangwagi-ro, Buk-gu, Gwangju, 61005, Republic of Korea.
National Nanofab Center, Korea Advanced Institute of Science and Technology, 291 Daehak-ro, Yuseong-gu, Daejeon, 34141, Republic of Korea.
Sci Rep. 2019 Mar 4;9(1):3350. doi: 10.1038/s41598-019-40001-1.
The engineering of structural colors is currently a promising, rapidly emerging research field because structural colors of outstanding spatial resolution and durability can be generated using a sustainable production method. However, the restricted and saturated color range in micro/nano-fabricated structural 'pigments' has hindered the dissemination of structural color printing. Here, this article presents a spectral mixing color filter (SMCF), which is the concept of fine-tunable color systems, capable of addressing the current issues in structural color engineering, by stacking a vertical silicon nanowire array embedded in a transparent polymer onto ultrathin optical coating layers. These two photonic structures enable independent tuning the optical resonance of each structure, depending on geometrical parameters, such as the diameter of nanowires and thickness of absorbing medium. Hence, the SMCF facilitates the linear combination of two resonant spectra, thereby enabling fine-tuning and widening of the color gamut. Theoretical studies and experimental results reveal the detailed working mechanisms and extraordinary mechanical feature of the SMCF. Based on the analyses, the concept of flexible optical device, e.g., a reflective anti-counterfeiting sticker, is demonstrated. Successful characterization demonstrates that the proposed strategy can promote the color controllability/purity of structural color and the applicability as flexible optical device.
结构色工程目前是一个很有前景、迅速兴起的研究领域,因为可以使用可持续生产方法生成具有出色空间分辨率和耐久性的结构色。然而,微纳制造的结构“颜料”中有限且饱和的色域阻碍了结构色印刷的推广。在此,本文提出了一种光谱混合滤色器(SMCF),它是一种精细可调颜色系统的概念,通过将嵌入透明聚合物中的垂直硅纳米线阵列堆叠到超薄光学涂层上,能够解决结构色工程中的当前问题。这两种光子结构能够根据几何参数(如纳米线直径和吸收介质厚度)独立调节每个结构的光学共振。因此,SMCF有助于两种共振光谱的线性组合,从而实现色域的精细调节和拓宽。理论研究和实验结果揭示了SMCF的详细工作机制和非凡的机械特性。基于这些分析,展示了柔性光学器件(如反射防伪贴纸)的概念。成功的表征表明,所提出的策略可以提高结构色的颜色可控性/纯度以及作为柔性光学器件的适用性。