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定制水凝胶的纳米级表面形貌以实现高效太阳能蒸汽产生。

Tailoring Nanoscale Surface Topography of Hydrogel for Efficient Solar Vapor Generation.

作者信息

Guo Youhong, Zhao Fei, Zhou Xingyi, Chen Zhichao, Yu Guihua

机构信息

Materials Science and Engineering Program and Department of Mechanical Engineering , The University of Texas at Austin , Austin , Texas 78712 , United States.

McKetta Department of Chemical Engineering , The University of Texas at Austin , Austin , Texas 78712 , United States.

出版信息

Nano Lett. 2019 Apr 10;19(4):2530-2536. doi: 10.1021/acs.nanolett.9b00252. Epub 2019 Mar 7.

Abstract

Solar vapor generation, which can separate the soluble or dispersing contaminants from water, is particularly desirable owing to its green energy utilization for water purification technology. Here, we present a concept of enhancing solar vapor generation by tailoring surface topography of the hydrogel-based solar evaporator. Via nanotexture-enhanced heat flux at the evaporation front, the obtained solar evaporator achieves a water evaporation rate of ∼2.6 kg m h at ∼91% energy efficiency under one sun (1 kW m). An easy-to-install solar still based on this solar evaporator consisting of cost-effective poly(vinyl alcohol) and activated carbon is deployed to demonstrate the potential for domestic or urgent water purification purposes. Such new design principles of hydrogel-based solar evaporators provides a useful means for surface-enhanced water evaporation to inspire scalable and processable solar evaporators from accessible raw materials.

摘要

太阳能蒸汽发生技术可将水中的可溶性或分散性污染物分离出来,因其在水净化技术中利用绿色能源而备受青睐。在此,我们提出了一种通过调整水凝胶基太阳能蒸发器的表面形貌来增强太阳能蒸汽发生的概念。通过蒸发前沿的纳米纹理增强热通量,所制备的太阳能蒸发器在一个太阳光照强度(1 kW/m²)下实现了约2.6 kg m⁻² h⁻¹的水蒸发速率,能量效率约为91%。基于这种由具有成本效益的聚乙烯醇和活性炭组成的太阳能蒸发器,我们部署了一种易于安装的太阳能蒸馏器,以展示其用于家庭或应急水净化的潜力。这种水凝胶基太阳能蒸发器的新设计原理为表面增强水蒸发提供了一种有用的方法,以激发利用易得原材料制备可扩展且可加工的太阳能蒸发器。

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