O Ramírez Mariola, Molina Pablo, Gómez-Tornero Alejandro, Hernández-Pinilla David, Sánchez-García Laura, Carretero-Palacios Sol, Bausá Luisa E
Departamento Física de Materiales, Instituto de Materiales Nicolás Cabrera and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, 28049, Madrid, Spain.
Adv Mater. 2019 Aug;31(35):e1901428. doi: 10.1002/adma.201901428. Epub 2019 Jun 27.
Coherent light sources providing sub-wavelength confined modes are in ever more demand to face new challenges in a variety of disciplines. Scalability and cost-effective production of these systems are also highly desired. The use of ferroelectrics in functional optical platforms, on which plasmonic arrangements can be formed, is revealed as a simple and powerful method to develop coherent light sources with improved and novel functionalities at the nanoscale. Two types of sources with sub-diffraction spatial confinement and improved performances are presented: i) plasmon-assisted solid-state nanolasers based on the interaction between metallic nanostructures and optically active rare earth doped ferroelectric crystals and ii) nonlinear radiation sources based on quadratic frequency mixing processes that are enhanced by means of localized surface plasmon (LSP) resonances. The mechanisms responsible for the intensification of the radiation-matter interaction processes by LSP resonances are discussed in each case. The challenges, potential applications, and future perspectives of the field are highlighted.
面对各学科中的新挑战,对提供亚波长受限模式的相干光源的需求日益增加。这些系统的可扩展性和具有成本效益的生产也备受期待。在功能性光学平台中使用铁电体(在其上可以形成等离子体排列),被证明是一种在纳米尺度上开发具有改进和新颖功能的相干光源的简单而强大的方法。本文介绍了两种具有亚衍射空间限制和改进性能的光源:i)基于金属纳米结构与光学活性稀土掺杂铁电晶体之间相互作用的等离子体辅助固态纳米激光器,以及ii)基于二次谐波混频过程的非线性辐射源,该过程通过局部表面等离子体(LSP)共振得到增强。每种情况下都讨论了由LSP共振导致辐射 - 物质相互作用过程增强的机制。文中强调了该领域的挑战、潜在应用和未来前景。