Liu Junting, Khayrudinov Vladislav, Yang He, Sun Yue, Matveev Boris, Remennyi Maxim, Yang Kejian, Haggren Tuomas, Lipsanen Harri, Wang Fengqiu, Zhang Baitao, He Jingliang
State Key Laboratory of Crystal Materials, Institute of Crystal Materials , Shandong University , Shandong , Jinan 250100 , China.
Department of Electronics and Nanoengineering , Aalto University , Espoo FI-00076 , Finland.
J Phys Chem Lett. 2019 Aug 1;10(15):4429-4436. doi: 10.1021/acs.jpclett.9b01626. Epub 2019 Jul 23.
Due to their tunable optical properties with various shapes, sizes, and compositions, nanowires (NWs) have been regarded as a class of semiconductor nanostructures with great potential for photodetectors, light-emitting diodes, gas sensors, microcavity lasers, optical modulators, and converters. Indium arsenide (InAs), an attractive III-V semiconductor NW with the advantages of narrow bandgap and large electron mobility, has attracted considerable interest in infrared optoelectronic and photonic devices. Here, we studied the ultrafast carrier dynamics and nonlinear optical responses of InAs NWs ranging from 1.0 to 2.8 μm and demonstrated the InAs-NW-based ultrafast broadband optical switch for passively Q-switching in all-solid-state laser systems. Furthermore, we achieved ultrafast optical modulation for laser mode-locking at 1.0 μm, paving the way for their applications in the field of ultrafast optics. These exotic optical properties indicate that InAs NWs have significant potential for various optoelectronic and photonic devices, especially in the mid-infrared wavelength range.
由于纳米线(NWs)具有可通过各种形状、尺寸和成分调节的光学特性,它们被视为一类在光电探测器、发光二极管、气体传感器、微腔激光器、光调制器和转换器等方面具有巨大潜力的半导体纳米结构。砷化铟(InAs)是一种具有吸引力的III-V族半导体纳米线,具有窄带隙和大电子迁移率的优点,在红外光电子和光子器件方面引起了相当大的兴趣。在此,我们研究了波长范围为1.0至2.8μm的InAs纳米线的超快载流子动力学和非线性光学响应,并展示了基于InAs纳米线的超快宽带光开关,用于全固态激光系统中的被动调Q。此外,我们实现了1.0μm激光锁模的超快光调制,为其在超快光学领域的应用铺平了道路。这些奇异的光学特性表明InAs纳米线在各种光电子和光子器件中具有巨大潜力,特别是在中红外波长范围内。