Faculty of Pharmacy in Hradec Králové , Charles University , Akademika Heyrovského 1203 , 50005 Hradec Králové , Czech Republic.
Faculty of Natural Sciences, Department of Biochemistry , Comenius University in Bratislava , Mlynská Dolina, Ilkovičova 6 , 842 15 Bratislava , Slovakia.
J Med Chem. 2019 Sep 12;62(17):8115-8139. doi: 10.1021/acs.jmedchem.9b00912. Epub 2019 Aug 22.
We report herein the discovery of 3,5-dinitrophenyl 1,2,4-triazoles with excellent and selective antimycobacterial activities against strains, including clinically isolated multidrug-resistant strains. Thorough structure-activity relationship studies of 3,5-dinitrophenyl-containing 1,2,4-triazoles and their trifluoromethyl analogues revealed the key role of the position of the 3,5-dinitrophenyl fragment in the antitubercular efficiency. Among the prepared compounds, the highest in vitro antimycobacterial activities against HRv and against seven clinically isolated multidrug-resistant strains of were found with S-substituted 4-alkyl-5-(3,5-dinitrophenyl)-4-1,2,4-triazole-3-thiols and their 3-nitro-5-(trifluoromethyl)phenyl analogues. The minimum inhibitory concentrations of these compounds reached 0.03 μM, which is superior to all the current first-line anti-tuberculosis drugs. Furthermore, almost all compounds with excellent antimycobacterial activities exhibited very low in vitro cytotoxicities against two proliferating mammalian cell lines. The docking study indicated that these compounds acted as the inhibitors of decaprenylphosphoryl-β-d-ribofuranose 2'-oxidase enzyme, which was experimentally confirmed by two independent radiolabeling experiments.
我们在此报告了具有优异和选择性抗分枝杆菌活性的 3,5-二硝基苯基 1,2,4-三唑的发现,包括临床分离的多药耐药株。对含 3,5-二硝基苯基的 1,2,4-三唑及其三氟甲基类似物的深入构效关系研究揭示了 3,5-二硝基苯基片段在抗结核效率中的关键作用。在所制备的化合物中,具有 S-取代的 4-烷基-5-(3,5-二硝基苯基)-4-1,2,4-三唑-3-硫醇及其 3-硝基-5-(三氟甲基)苯基类似物对 HRv 和七种临床分离的多药耐药株的体外抗分枝杆菌活性最高。这些化合物的最低抑菌浓度达到 0.03 μM,优于所有当前的一线抗结核药物。此外,几乎所有具有优异抗分枝杆菌活性的化合物对两种增殖的哺乳动物细胞系的体外细胞毒性都非常低。对接研究表明,这些化合物作为脱磷酸化-β-d-核糖呋喃糖 2'-氧化酶的抑制剂,这通过两个独立的放射性标记实验得到了实验证实。