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磁场中规则/不规则平面量子点的强关联激子:通过多极展开的尺寸广延双激子和三激子(电子 - 空穴 - 电子 - 空穴和电子 - 电子 - 空穴/电子 - 空穴 - 空穴)系统

Strongly Correlated Excitons of Regular/Irregular Planar Quantum Dots in Magnetic Field: Size-Extensive Bi- and Triexciton (e-h-e-h and e-e-h/e-h-h) Systems by Multipole Expansion.

作者信息

Kaur Harsimran, Singh Sunny, Aggarwal Priyanka, Sharma Shivalika, Yadav Sambhav, Hazra Ram Kuntal

机构信息

Department of Chemistry (Physical), University of Delhi, Vishwavidyalaya Marg, North Campus, 110 007 New Delhi, India.

出版信息

ACS Omega. 2017 Oct 31;2(10):7410-7423. doi: 10.1021/acsomega.7b00886.

Abstract

Excitons in parabolically confined planar quantum dots with a transverse magnetic field have been studied in various model systems. The correlations between e-h, e-e, and h-h have been incorporated in terms of exact, simply elegant, and absolutely terminating finite summed Lauricella functions which eliminate the secular divergence problem and pave way for a comprehensive understanding of certain exotic phenomena of various two-dimensional regular and irregular quantum dots. A simple yet highly accurate and exact variational wave function in terms of Whittaker- function extensible to multiexcitonic systems has been propounded. We have also presented a formulation extending the size of the systems to triexcitonic (e-e-h/e-h-h), biexcitonic (e-h-e-h), and multiexcitonic ("N" e-h pair) planar dots by mono-, di-, quadru-, and octopole expansions. As a benchmark, we have examined the energy spectra, level-spacing statistics, heat capacities ( at 1 K), and magnetization ( ≈ 0-1 K) of He/SiO/BN/GaAs model systems for different lateral confinements, magnetic fields, mass ratios of e-h, and dielectric constants (ϵ).

摘要

在各种模型系统中,对具有横向磁场的抛物线型受限平面量子点中的激子进行了研究。电子 - 空穴(e - h)、电子 - 电子(e - e)和空穴 - 空穴(h - h)之间的相关性已通过精确、简洁且绝对收敛的有限求和劳里切拉函数纳入,这些函数消除了长期发散问题,并为全面理解各种二维规则和不规则量子点的某些奇异现象铺平了道路。提出了一种基于惠特克函数的简单但高度准确且精确的变分波函数,该函数可扩展到多激子系统。我们还提出了一种通过单极、偶极、四极和八极展开将系统尺寸扩展到三激子(e - e - h / e - h - h)、双激子(e - h - e - h)和多激子(“N”个e - h对)平面量子点的公式。作为基准,我们研究了He/SiO/BN/GaAs模型系统在不同横向限制、磁场、e - h质量比和介电常数(ϵ)下的能谱、能级间距统计、热容量(在1 K时)和磁化强度(≈0 - 1 K)。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1132/6645354/55a32466093c/ao-2017-00886y_0001.jpg

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