Suppr超能文献

等离子体纳米尖峰的光热效应用于 LSPR 传感。

Photothermal Effect in Plasmonic Nanotip for LSPR Sensing.

机构信息

State Key Laboratory of Bioelectronics, School of Biological Science and Medical Engineering, Southeast University, Nanjing 210096, China.

Southeast University-Shenzhen Research Institute, Shenzhen 518000, China.

出版信息

Sensors (Basel). 2020 Jan 25;20(3):671. doi: 10.3390/s20030671.

Abstract

The influence of heat generation on the conventional process of LSPR based sensing has not been explored thus far. Therefore, a need exists to draw attention toward the heat generation issue during LSPR sensing as it may affect the refractive index of the analyte, leading to incorrect sensory conclusions. This manuscript addresses the connection between the photo-thermal effect and LSPR. We numerically analyzed the heat performance of a gold cladded nanotip. The numerical results predict a change in the micro-scale temperature in the microenvironment near the nanotip. These numerical results predict a temperature increase of more than 20 K near the apex of the nanotip, which depends on numerous factors including the input optical power and the diameter of the fiber. We analytically show that this change in the temperature influences a change in the refractive index of the microenvironment in the vicinity of the nanotip. In accordance with our numerical and analytical findings, we experimentally show an LSPR shift induced by a change in the input power of the source. We believe that our work will bring the importance of temperature dependence in nanotip based LSPR sensing to the fore.

摘要

迄今为止,尚未探究发热对基于局域表面等离子体共振(LSPR)的传统传感过程的影响。因此,需要关注 LSPR 传感过程中的发热问题,因为它可能会影响分析物的折射率,导致错误的传感结论。本文探讨了光热效应与 LSPR 之间的联系。我们对金覆盖纳米尖端的热性能进行了数值分析。数值结果预测了纳米尖端附近微环境中微尺度温度的变化。这些数值结果预测在纳米尖端的顶点附近温度会升高 20K 以上,这取决于包括输入光功率和光纤直径在内的众多因素。我们从理论上证明了这种温度变化会影响纳米尖端附近微环境的折射率变化。根据我们的数值和分析结果,我们实验展示了由光源输入功率变化引起的 LSPR 位移。我们相信,我们的工作将使基于纳米尖端的 LSPR 传感中温度依赖性的重要性得到突显。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a783/7039235/9d93f918c767/sensors-20-00671-g001.jpg

文献AI研究员

20分钟写一篇综述,助力文献阅读效率提升50倍。

立即体验

用中文搜PubMed

大模型驱动的PubMed中文搜索引擎

马上搜索

文档翻译

学术文献翻译模型,支持多种主流文档格式。

立即体验