Flöry Nikolaus, Ma Ping, Salamin Yannick, Emboras Alexandros, Taniguchi Takashi, Watanabe Kenji, Leuthold Juerg, Novotny Lukas
Photonics Laboratory, ETH Zürich, Zurich, Switzerland.
Institute of Electromagnetic Fields, ETH Zürich, Zurich, Switzerland.
Nat Nanotechnol. 2020 Feb;15(2):118-124. doi: 10.1038/s41565-019-0602-z. Epub 2020 Feb 3.
Intensive efforts have been devoted to the exploration of new optoelectronic devices based on two-dimensional transition-metal dichalcogenides (TMDCs) owing to their strong light-matter interaction and distinctive material properties. In particular, photodetectors featuring both high-speed and high-responsivity performance are of great interest for a vast number of applications such as high-data-rate interconnects operated at standardized telecom wavelengths. Yet, the intrinsically small carrier mobilities of TMDCs become a bottleneck for high-speed application use. Here, we present high-performance vertical van der Waals heterostructure-based photodetectors integrated on a silicon photonics platform. Our vertical MoTe-graphene heterostructure design minimizes the carrier transit path length in TMDCs and enables a record-high measured bandwidth of at least 24 GHz under a moderate bias voltage of -3 V. Applying a higher bias or employing thinner MoTe flakes boosts the bandwidth even to 50 GHz. Simultaneously, our device reaches a high external responsivity of 0.2 A W for incident light at 1,300 nm, benefiting from the integrated waveguide design. Our studies shed light on performance trade-offs and present design guidelines for fast and efficient devices. The combination of two-diemensional heterostructures and integrated guided-wave nano photonics defines an attractive platform to realize high-performance optoelectronic devices, such as photodetectors, light-emitting devices and electro-optic modulators.
由于二维过渡金属二硫属化物(TMDCs)具有强光与物质相互作用以及独特的材料特性,人们一直致力于探索基于它们的新型光电器件。特别是,兼具高速和高响应性能的光电探测器在众多应用中备受关注,例如在标准电信波长下运行的高数据速率互连。然而,TMDCs固有的小载流子迁移率成为高速应用的瓶颈。在此,我们展示了集成在硅光子学平台上的基于高性能垂直范德华异质结构的光电探测器。我们的垂直MoTe-石墨烯异质结构设计使TMDCs中的载流子传输路径长度最小化,并在-3 V的适度偏置电压下实现了创纪录的至少24 GHz的测量带宽。施加更高的偏置或使用更薄的MoTe薄片可将带宽提高到50 GHz。同时,得益于集成波导设计,我们的器件对1300 nm的入射光达到了0.2 A W的高外部响应度。我们的研究揭示了性能权衡,并为快速高效的器件提供了设计指南。二维异质结构与集成光波导纳米光子学的结合定义了一个有吸引力的平台,可用于实现高性能光电器件,如光电探测器、发光器件和电光调制器。