Xue Yongzhou, Wang Hui, Xie Nan, Yang Qian, Xu Fujun, Shen Bo, Shi Jun-Jie, Jiang Desheng, Dou Xiuming, Yu Tongjun, Sun Bao-Quan
State Key Laboratory for Superlattices and Microstructures, Institute of Semiconductors, Chinese Academy of Sciences, Beijing 100083, China.
State Key Laboratory for Artificial Microstructures and Mesoscopic Physics, School of Physics, Peking University, Beijing 100871, China.
J Phys Chem Lett. 2020 Apr 2;11(7):2689-2694. doi: 10.1021/acs.jpclett.0c00511. Epub 2020 Mar 23.
Quantum technologies require robust and photostable single-photon emitters. Here, room temperature operated single-photon emissions from isolated defects in aluminum nitride (AlN) films are reported. AlN films were grown on nanopatterned sapphire substrates by metal organic chemical vapor deposition. The observed emission lines range from visible to near-infrared, with highly linear polarization characteristics. The temperature-dependent line width increase shows T or single-exponential behavior. First-principle calculations based on density functional theory show that point defect species, such as antisite nitrogen vacancy complex (NV) and divacancy (VV) complexes, are considered to be an important physical origin of observed emission lines ranging from approximately 550 to 1000 nm. The results provide a new platform for on-chip quantum sources.
量子技术需要坚固且光稳定的单光子发射器。在此,报道了氮化铝(AlN)薄膜中孤立缺陷在室温下的单光子发射。通过金属有机化学气相沉积在纳米图案蓝宝石衬底上生长AlN薄膜。观察到的发射线范围从可见光到近红外,具有高度线性偏振特性。温度依赖性线宽增加呈现出T或单指数行为。基于密度泛函理论的第一性原理计算表明,诸如反位氮空位复合体(NV)和双空位(VV)复合体等点缺陷物种被认为是观察到的约550至1000nm发射线的重要物理起源。这些结果为片上量子源提供了一个新平台。