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六方氮化硼单层中的量子发射。

Quantum emission from hexagonal boron nitride monolayers.

机构信息

School of Mathematical and Physical Sciences, University of Technology Sydney, Ultimo, New South Wales 2007, Australia.

出版信息

Nat Nanotechnol. 2016 Jan;11(1):37-41. doi: 10.1038/nnano.2015.242. Epub 2015 Oct 26.

Abstract

Artificial atomic systems in solids are widely considered the leading physical system for a variety of quantum technologies, including quantum communications, computing and metrology. To date, however, room-temperature quantum emitters have only been observed in wide-bandgap semiconductors such as diamond and silicon carbide, nanocrystal quantum dots, and most recently in carbon nanotubes. Single-photon emission from two-dimensional materials has been reported, but only at cryogenic temperatures. Here, we demonstrate room-temperature, polarized and ultrabright single-photon emission from a colour centre in two-dimensional hexagonal boron nitride. Density functional theory calculations indicate that vacancy-related defects are a probable source of the emission. Our results demonstrate the unprecedented potential of van der Waals crystals for large-scale nanophotonics and quantum information processing.

摘要

人工原子系统在固体中被广泛认为是各种量子技术的主要物理系统,包括量子通信、计算和计量学。然而,迄今为止,室温量子发射器仅在宽带隙半导体如金刚石和碳化硅、纳米晶体量子点中,以及最近在碳纳米管中观察到。已经报道了二维材料的单光子发射,但仅在低温下。在这里,我们展示了来自二维六方氮化硼中色心的室温、极化和超高亮度的单光子发射。密度泛函理论计算表明,与空位相关的缺陷可能是发射的来源。我们的结果表明,范德华晶体在大规模纳米光子学和量子信息处理方面具有前所未有的潜力。

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