Sriram Pavithra, Manikandan Arumugam, Chuang Feng-Chuan, Chueh Yu-Lun
Department of Materials Science and Engineering, National Tsing Hua University, Hsinchu, 30013, Taiwan.
Department of Physics, National Sun Yat-Sen University, Kaohsiung, 80424, Taiwan.
Small. 2020 Apr;16(15):e1904271. doi: 10.1002/smll.201904271. Epub 2020 Mar 20.
Recently, 2D transition metal dichalcogenides (TMDs) have become intriguing materials in the versatile field of photonics and optoelectronics because of their strong light-matter interaction that stems from the atomic layer thickness, broadband optical response, controllable optoelectronic properties, and high nonlinearity, as well as compatibility. Nevertheless, the low optical cross-section of 2D-TMDs inhibits the light-matter interaction, resulting in lower quantum yield. Therefore, hybridizing the 2D-TMDs with plasmonic nanomaterials has become one of the promising strategies to boost the optical absorption of thin 2D-TMDs. The appeal of plasmonics is based on their capability to localize and enhance the electromagnetic field and increase the optical path length of light by scattering and injecting hot electrons to TMDs. In this regard, recent achievements with respect to hybridization of the plasmonic effect in 2D-TMDs systems and its augmented optical and optoelectronic properties are reviewed. The phenomenon of plasmon-enhanced interaction in 2D-TMDs is briefly described and state-of-the-art hybrid device applications are comprehensively discussed. Finally, an outlook on future applications of these hybrid devices is provided.
近年来,二维过渡金属二硫属化物(TMDs)因其源于原子层厚度的强光与物质相互作用、宽带光学响应、可控的光电特性、高非线性以及兼容性,在光子学和光电子学的广泛领域中成为引人关注的材料。然而,二维TMDs的低光学截面抑制了光与物质的相互作用,导致量子产率较低。因此,将二维TMDs与等离子体纳米材料杂交已成为提高二维薄TMDs光吸收的一种有前景的策略。等离子体激元学的吸引力基于其能够通过散射并向TMDs注入热电子来局域化和增强电磁场以及增加光的光程长度。在此方面,本文综述了二维TMDs系统中等离子体激元效应杂交及其增强的光学和光电特性的近期研究成果。简要描述了二维TMDs中等离子体激元增强相互作用的现象,并全面讨论了最新的混合器件应用。最后,对这些混合器件的未来应用进行了展望。