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中红外飞秒激光脉冲作用下电介质中的电离过程及激光诱导周期性表面结构

Ionisation processes and laser induced periodic surface structures in dielectrics with mid-infrared femtosecond laser pulses.

作者信息

Tsibidis George D, Stratakis Emmanuel

机构信息

Institute of Electronic Structure and Laser (IESL), Foundation for Research and Technology (FORTH), N. Plastira 100, Vassilika Vouton, 70013, Heraklion, Crete, Greece.

Department of Physics, University of Crete, 71003, Heraklion, Greece.

出版信息

Sci Rep. 2020 May 26;10(1):8675. doi: 10.1038/s41598-020-65613-w.

DOI:10.1038/s41598-020-65613-w
PMID:32457397
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7250856/
Abstract

Irradiation of solids with ultrashort pulses and laser processing in the mid-Infrared (mid-IR) spectral region is a yet predominantly unexplored field with a large potential for a wide range of applications. In this work, laser driven physical phenomena associated with processes following irradiation of fused silica (SiO) with ultrashort laser pulses in the mid-IR region are investigated in detail. A multiscale modelling approach is performed that correlates conditions for formation of perpendicular or parallel to the laser polarisation low spatial frequency periodic surface structures for low and high intensity mid-IR pulses (not previously explored in dielectrics at those wavelengths), respectively. Results demonstrate a remarkable domination of tunneling effects in the photoionisation rate and a strong influence of impact ionisation for long laser wavelengths. The methodology presented in this work is aimed to shed light on the fundamental mechanisms in a previously unexplored spectral area and allow a systematic novel surface engineering with strong mid-IR fields for advanced industrial laser applications.

摘要

用超短脉冲对固体进行辐照以及在中红外(mid - IR)光谱区域进行激光加工,是一个尚未得到充分探索的领域,具有广泛应用的巨大潜力。在这项工作中,详细研究了与在中红外区域用超短激光脉冲辐照熔融石英(SiO)后发生的过程相关的激光驱动物理现象。采用了一种多尺度建模方法,该方法分别关联了低强度和高强度中红外脉冲(在那些波长下,电介质中此前尚未探索过)形成与激光偏振垂直或平行的低空间频率周期性表面结构的条件。结果表明,在光电离速率中隧道效应占显著主导地位,并且对于长激光波长,碰撞电离有很强的影响。这项工作中提出的方法旨在揭示一个此前未探索光谱区域的基本机制,并允许利用强中红外场进行系统的新型表面工程,以用于先进的工业激光应用。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/9a39202a31ac/41598_2020_65613_Fig8_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/a17a3b23804a/41598_2020_65613_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/d53da5a9250b/41598_2020_65613_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/56dbfcc154b6/41598_2020_65613_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/7704a63e2a1d/41598_2020_65613_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/65040db5bdfd/41598_2020_65613_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/4828d6b0bb9e/41598_2020_65613_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/55a930134783/41598_2020_65613_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/9a39202a31ac/41598_2020_65613_Fig8_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/a17a3b23804a/41598_2020_65613_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/d53da5a9250b/41598_2020_65613_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/56dbfcc154b6/41598_2020_65613_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/7704a63e2a1d/41598_2020_65613_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/65040db5bdfd/41598_2020_65613_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/4828d6b0bb9e/41598_2020_65613_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/55a930134783/41598_2020_65613_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/432e/7250856/9a39202a31ac/41598_2020_65613_Fig8_HTML.jpg

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本文引用的文献

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Single-Shot Multi-Stage Damage and Ablation of Silicon by Femtosecond Mid-infrared Laser Pulses.飞秒中红外激光脉冲对硅的单次多阶段损伤与烧蚀
Sci Rep. 2019 Dec 27;9(1):19993. doi: 10.1038/s41598-019-56384-0.
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Biomimetic Omnidirectional Antireflective Glass via Direct Ultrafast Laser Nanostructuring.通过直接超快激光纳米结构化制备的仿生全向抗反射玻璃
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二维钛铁多层凝聚体上的飞秒激光诱导周期性表面结构
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