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二维钛铁多层凝聚体上的飞秒激光诱导周期性表面结构

Femtosecond Laser-Induced Periodic Surface Structures on 2D Ti-Fe Multilayer Condensates.

作者信息

Kuznietsov Oleksandr V, Tsibidis George D, Demchishin Anatoliy V, Demchishin Anatoliy A, Babizhetskyy Volodymyr, Saldan Ivan, Bellucci Stefano, Gnilitskyi Iaroslav

机构信息

NoviNano Lab LLC, Pasternaka 5, 79015 Lviv, Ukraine.

Department of Photonics, Lviv Polytechnic National University, 79013 Lviv, Ukraine.

出版信息

Nanomaterials (Basel). 2021 Jan 27;11(2):316. doi: 10.3390/nano11020316.

DOI:10.3390/nano11020316
PMID:33513705
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7911909/
Abstract

2D Ti-Fe multilayer preparation has been attracting increased interest due to its ability to form intermetallic compounds between metallic titanium and metallic iron thin layers. In particular, the TiFe compound can absorb hydrogen gas at room temperature. We applied femtosecond laser pulses to heat Ti-Fe multilayer structures to promote the appearance of intermetallic compounds and generate surface nanostructuring. The surface pattern, known as Laser Induced Periodic Surface Structures (LIPSS), can accelerate the kinetics of chemical interaction between solid TiFe and gaseous hydrogen. The formation of LIPSS on Ti-Fe multilayered thin films were investigated using of scanning electron microscopy, photo-electron spectroscopy and X-ray diffraction. To explore the thermal response of the multiple layered structure and the mechanisms leading to surface patterning after irradiating the compound with single laser pulses, theoretical simulations were conducted to interpret the experimental observations.

摘要

二维钛铁多层膜的制备因其能够在金属钛和金属铁薄层之间形成金属间化合物而越来越受到关注。特别是，TiFe化合物在室温下能吸收氢气。我们应用飞秒激光脉冲加热Ti-Fe多层结构，以促进金属间化合物的出现并产生表面纳米结构。这种被称为激光诱导周期性表面结构（LIPSS）的表面图案可以加速固态TiFe和气态氢之间的化学相互作用动力学。利用扫描电子显微镜、光电子能谱和X射线衍射研究了Ti-Fe多层薄膜上LIPSS的形成。为了探索多层结构的热响应以及在用单个激光脉冲照射该化合物后导致表面图案化的机制，进行了理论模拟以解释实验观察结果。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/22cd19bd45fb/nanomaterials-11-00316-g005a.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/d12629246911/nanomaterials-11-00316-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/fda3aef6bd9f/nanomaterials-11-00316-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/ebf682554073/nanomaterials-11-00316-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/86adc7c9b171/nanomaterials-11-00316-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/22cd19bd45fb/nanomaterials-11-00316-g005a.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/d12629246911/nanomaterials-11-00316-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/fda3aef6bd9f/nanomaterials-11-00316-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/ebf682554073/nanomaterials-11-00316-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/86adc7c9b171/nanomaterials-11-00316-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e7ee/7911909/22cd19bd45fb/nanomaterials-11-00316-g005a.jpg

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