State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Beijing Normal University, Beijing 100875, China.
State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Beijing Normal University, Beijing 100875, China.
Sci Total Environ. 2020 Nov 1;741:140191. doi: 10.1016/j.scitotenv.2020.140191. Epub 2020 Jun 16.
Nitrogen deposition in lake sediment is an important factor reflecting the evolution of lake environments. Over the past 150-200 years, lakes in China have been affected by natural factors and anthropogenic factors, and nitrogen deposition has increased. As a result, it is critical to reconstruct the spatiotemporal variation trend of nitrogen deposition and analyse the nitrogen source and driving factors. On a regional scale, based on the sediment TN, δN and C: N ratio variation trends, this study analysed the buried nitrogen variation trend in Yunnan-Guizhou Plateau lakes over the past 150-200 years. The effects of lake morphology on nitrogen deposition were also analysed by using natural lake parameters. At the watershed scale, the δN isotope in the sediment was used to distinguish the sediment sources. On this basis, this study analysed the relationship between nitrogen deposition in nine lakes and the socioeconomic conditions during 1949-2010. The results show that (1) during the last 150-200 years, the TN, δN and the C: N ratio in the sediments increased. (2) Lake depth and area are the main natural factors affecting the extent of nitrogen deposition. (3) Before 1950, the nitrogen in the lake sediments in the region was sourced mainly from natural sources such as precipitation, woodland, grassland and aquatic plants. After 1950, man-made sources such as sewage and farmland became the main sources of nitrogen. (4) Human social and economic activities have an increasingly significant influence on the lake water environment in the Yunnan-Guizhou Plateau and are also the main factors leading to the deterioration of the aquatic environment.
湖泊沉积物中的氮沉积是反映湖泊环境演化的一个重要因素。过去 150-200 年来,中国的湖泊受到自然因素和人为因素的影响,氮沉积增加。因此,重建氮沉积的时空变化趋势,分析氮的来源和驱动因素至关重要。在区域尺度上,本研究基于湖泊沉积物总氮(TN)、δN 和 C:N 比值的变化趋势,分析了过去 150-200 年来云贵高原湖泊埋藏氮的变化趋势。同时,利用自然湖泊参数分析了湖泊形态对氮沉积的影响。在流域尺度上,利用沉积物中的δN 同位素来区分沉积物来源。在此基础上,分析了 1949-2010 年期间 9 个湖泊氮沉积与社会经济条件之间的关系。结果表明:(1)过去 150-200 年来,沉积物中的 TN、δN 和 C:N 比值增加;(2)湖深和面积是影响氮沉积程度的主要自然因素;(3)1950 年以前,该地区湖泊沉积物中的氮主要来源于降水、林地、草地和水生植物等自然源,1950 年以后,污水和农田等人为源成为氮的主要来源;(4)人类社会经济活动对云贵高原湖泊水环境的影响日益显著,也是导致水环境污染恶化的主要因素。