Kvashnin Y, VanGennep D, Mito M, Medvedev S A, Thiyagarajan R, Karis O, Vasiliev A N, Eriksson O, Abdel-Hafiez M
Uppsala University, Department of Physics and Astronomy, Box 516, SE-751 20 Uppsala, Sweden.
Lyman Laboratory of Physics, Harvard University, Cambridge, Massachusetts 02138, USA.
Phys Rev Lett. 2020 Oct 30;125(18):186401. doi: 10.1103/PhysRevLett.125.186401.
The coexistence of charge density wave (CDW) and superconductivity in tantalum disulfide (2H-TaS_{2}) at low temperature is boosted by applying hydrostatic pressures to study both vibrational and magnetic transport properties. Around P_{c}, we observe a superconducting dome with a maximum superconducting transition temperature T_{c}=9.1 K. First-principles calculations of the electronic structure predict that, under ambient conditions, the undistorted structure is characterized by a phonon instability at finite momentum close to the experimental CDW wave vector. Upon compression, this instability is found to disappear, indicating the suppression of CDW order. The calculations reveal an electronic topological transition (ETT), which occurs before the suppression of the phonon instability, suggesting that the ETT alone is not directly causing the structural change in the system. The temperature dependence of the first vortex penetration field has been experimentally obtained by two independent methods. While a d wave and single-gap BCS prediction cannot describe the lower critical field H_{c1} data, the temperature dependence of the H_{c1} can be well described by a single-gap anisotropic s-wave order parameter.
通过施加静水压力来研究二硫化钽(2H-TaS₂)在低温下电荷密度波(CDW)与超导性的共存情况,这推动了对其振动和磁输运性质的研究。在Pc附近,我们观察到一个超导圆顶,其最大超导转变温度Tc = 9.1 K。电子结构的第一性原理计算预测,在环境条件下,未畸变结构的特征是在接近实验CDW波矢的有限动量处存在声子不稳定性。压缩时,发现这种不稳定性消失,表明CDW序被抑制。计算揭示了一个电子拓扑转变(ETT),它发生在声子不稳定性被抑制之前,这表明单独的ETT并非直接导致系统结构变化。通过两种独立方法实验获得了第一个涡旋穿透场的温度依赖性。虽然d波和单能隙BCS预测无法描述下临界场Hc1数据,但单能隙各向异性s波序参量可以很好地描述Hc1的温度依赖性。