Department of Applied Physics and Applied Mathematics, Columbia University, New York, New York 10027, United States.
Department of Chemistry, Columbia University, New York, New York 10027, United States.
Nano Lett. 2020 Dec 9;20(12):8912-8918. doi: 10.1021/acs.nanolett.0c03994. Epub 2020 Nov 18.
Light emission from tunnel junctions are a potential photon source for nanophotonic applications. Surprisingly, the photons emitted can have energies exceeding the energy supplied to the electrons by the bias. Three mechanisms for generating these so-called overbias photons have been proposed, but the relationship between these mechanisms has not been clarified. In this work, we argue that multielectron processes provide the best framework for understanding overbias light emission in tunnel junctions. Experimentally, we demonstrate for the first time that the superlinear dependence of emission on conductance predicted by this theory is robust to the temperature of the tunnel junction, indicating that tunnel junctions are a promising candidate for electrically driven broadband photon sources.
从隧道结中发射的光,是纳米光子学应用的一个潜在光子源。令人惊讶的是,发射出的光子的能量可以超过偏置施加到电子上的能量。已经提出了三种产生这些所谓过偏压光子的机制,但这些机制之间的关系尚未阐明。在这项工作中,我们认为多电子过程为理解隧道结中的过偏压光发射提供了最佳框架。实验上,我们首次证明了该理论预测的发射对电导的超线性依赖关系在隧道结温度下是稳健的,这表明隧道结是一种很有前途的电驱动宽带光子源的候选者。