Dai Wei, Wang Yujie, Li Ruixue, Fan Yubin, Qu Geyang, Wu Yunkai, Song Qinghai, Han Jiecai, Xiao Shumin
Ministry of Industry and Information Technology Key Lab of Micro-Nano Optoelectronic Information System, Harbin Institute of Technology (Shenzhen), Shenzhen 518055, China.
Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, China.
ACS Nano. 2020 Dec 22;14(12):17063-17070. doi: 10.1021/acsnano.0c06463. Epub 2020 Nov 24.
Micro- and nanolasers are miniaturized light sources with great potential in optical imaging, sensing, and communication. While various micro- and nanolasers have been synthesized, they are mostly linearly polarized and thus strongly restricted in many new applications, .., chiral resolution in synthetic chemistry, cancerous tissue imaging, information storage, and processing. Herein, we experimentally demonstrate the circularly polarized surface emitting perovskite lasers by integrating the as-grown perovskite microcrystals with an all-dielectric metalens. The perovskite microcrystal serves as an optical microcavity and produces linearly polarized laser emission, which is collected by a geometric phase based TiO metalens. The left-handed circularly polarized components are collimated by the metalens into a directional laser beam with a divergent angle of <0.9°, whereas the right-handed components are strongly diverged by the same metalens. Consequently, the right-handed circularly polarized components are filtered out, and perovskite lasers with high directionality and pure circular polarization have been experimentally realized.
微纳激光器是一种小型化光源,在光学成像、传感和通信领域具有巨大潜力。虽然已经合成了各种微纳激光器,但它们大多是线偏振的,因此在许多新应用中受到很大限制,……,如合成化学中的手性拆分、癌组织成像、信息存储和处理等。在此,我们通过将生长的钙钛矿微晶与全介质超表面透镜集成,实验证明了圆偏振表面发射钙钛矿激光器。钙钛矿微晶用作光学微腔并产生线偏振激光发射,该发射由基于几何相位的TiO超表面透镜收集。左旋圆偏振分量被超表面透镜准直成发散角<0.9°的定向激光束,而右旋分量被同一超表面透镜强烈发散。因此,右旋圆偏振分量被滤除,实验实现了具有高方向性和纯圆偏振的钙钛矿激光器。