Ravikumar Dwarakanath, Zhang Duo, Keoleian Gregory, Miller Shelie, Sick Volker, Li Victor
Center for Sustainable Systems (CSS), School for Environment and Sustainability (SEAS), University of Michigan, Ann Arbor, MI, USA.
National Renewable Energy Laboratory (NREL), Golden, CO, USA.
Nat Commun. 2021 Feb 8;12(1):855. doi: 10.1038/s41467-021-21148-w.
Carbon capture and utilization for concrete production (CCU concrete) is estimated to sequester 0.1 to 1.4 gigatons of carbon dioxide (CO) by 2050. However, existing estimates do not account for the CO impact from the capture, transport and utilization of CO, change in compressive strength in CCU concrete and uncertainty and variability in CCU concrete production processes. By accounting for these factors, we determine the net CO benefit when CCU concrete produced from CO curing and mixing substitutes for conventional concrete. The results demonstrate a higher likelihood of the net CO benefit of CCU concrete being negative i.e. there is a net increase in CO in 56 to 68 of 99 published experimental datasets depending on the CO source. Ensuring an increase in compressive strength from CO curing and mixing and decreasing the electricity used in CO curing are promising strategies to increase the net CO benefit from CCU concrete.
用于混凝土生产的碳捕获与利用(CCU混凝土)预计到2050年可封存0.1至1.4吉吨二氧化碳(CO₂)。然而,现有估算未考虑CO₂捕获、运输和利用过程中的CO₂影响、CCU混凝土抗压强度的变化以及CCU混凝土生产过程中的不确定性和变异性。通过考虑这些因素,我们确定了用CO₂养护和搅拌生产的CCU混凝土替代传统混凝土时的净CO₂效益。结果表明,CCU混凝土净CO₂效益为负的可能性更高,即根据CO₂来源,在99个已发表的实验数据集中,有56至68个数据集的CO₂净增加。确保CO₂养护和搅拌能提高抗压强度,并减少CO₂养护中所用电能,是增加CCU混凝土净CO₂效益的有前景的策略。