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锑化铟碲作为用于红外的可编程纳米光子学材料平台。

InSbTe as a programmable nanophotonics material platform for the infrared.

作者信息

Heßler Andreas, Wahl Sophia, Leuteritz Till, Antonopoulos Antonios, Stergianou Christina, Schön Carl-Friedrich, Naumann Lukas, Eicker Niklas, Lewin Martin, Maß Tobias W W, Wuttig Matthias, Linden Stefan, Taubner Thomas

机构信息

Institute of Physics (IA), RWTH Aachen University, Aachen, Germany.

Physikalisches Institut, University of Bonn, Bonn, Germany.

出版信息

Nat Commun. 2021 Feb 10;12(1):924. doi: 10.1038/s41467-021-21175-7.

Abstract

The high dielectric optical contrast between the amorphous and crystalline structural phases of non-volatile phase-change materials (PCMs) provides a promising route towards tuneable nanophotonic devices. Here, we employ the next-generation PCM InSbTe (IST) whose optical properties change from dielectric to metallic upon crystallization in the whole infrared spectral range. This distinguishes IST as a switchable infrared plasmonic PCM and enables a programmable nanophotonics material platform. We show how resonant metallic nanostructures can be directly written, modified and erased on and below the meta-atom level in an IST thin film by a pulsed switching laser, facilitating direct laser writing lithography without need for cumbersome multi-step nanofabrication. With this technology, we demonstrate large resonance shifts of nanoantennas of more than 4 µm, a tuneable mid-infrared absorber with nearly 90% absorptance as well as screening and nanoscale "soldering" of metallic nanoantennas. Our concepts can empower improved designs of programmable nanophotonic devices for telecommunications, (bio)sensing and infrared optics, e.g. programmable infrared detectors, emitters and reconfigurable holograms.

摘要

非易失性相变材料(PCM)的非晶态和晶态结构相之间的高介电光学对比度为可调谐纳米光子器件提供了一条很有前景的途径。在此,我们采用下一代PCM铟锑碲(IST),其在整个红外光谱范围内结晶时光学性质从介电转变为金属。这使IST成为一种可切换的红外等离子体PCM,并实现了一个可编程的纳米光子材料平台。我们展示了如何通过脉冲开关激光在IST薄膜的亚原子水平及以下直接写入、修改和擦除共振金属纳米结构,从而无需繁琐的多步纳米制造即可实现直接激光写入光刻。利用这项技术,我们展示了纳米天线超过4微米的大共振位移、具有近90%吸收率的可调谐中红外吸收器以及金属纳米天线的屏蔽和纳米级“焊接”。我们的概念能够推动用于电信、(生物)传感和红外光学的可编程纳米光子器件的改进设计,例如可编程红外探测器、发射器和可重构全息图。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e73/7876017/096cd8fd5e7a/41467_2021_21175_Fig1_HTML.jpg

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