Gilbert Dustin A, Murray Peyton D, De Rojas Julius, Dumas Randy K, Davies Joseph E, Liu Kai
Department of Materials Science and Engineering, University of Tennessee, Knoxville, TN, 37919, USA.
Department of Physics and Astronomy, University of Tennessee, Knoxville, TN, 37919, USA.
Sci Rep. 2021 Feb 17;11(1):4018. doi: 10.1038/s41598-021-83349-z.
The first order reversal curve (FORC) method is a magnetometry based technique used to capture nanoscale magnetic phase separation and interactions with macroscopic measurements using minor hysteresis loop analysis. This makes the FORC technique a powerful tool in the analysis of complex systems which cannot be effectively probed using localized techniques. However, recovering quantitative details about the identified phases which can be compared to traditionally measured metrics remains an enigmatic challenge. We demonstrate a technique to reconstruct phase-resolved magnetic hysteresis loops by selectively integrating the measured FORC distribution. From these minor loops, the traditional metrics-including the coercivity and saturation field, and the remanent and saturation magnetization-can be determined. In order to perform this analysis, special consideration must be paid to the accurate quantitative management of the so-called reversible features. This technique is demonstrated on three representative materials systems, high anisotropy FeCuPt thin-films, Fe nanodots, and SmCo/Fe exchange spring magnet films, and shows excellent agreement with the direct measured major loop, as well as the phase separated loops.
一阶反转曲线(FORC)方法是一种基于磁力测量的技术,通过小磁滞回线分析,利用宏观测量来捕捉纳米级磁相分离和相互作用。这使得FORC技术成为分析复杂系统的有力工具,而这些复杂系统无法用局部技术进行有效探测。然而,恢复关于已识别相的定量细节,以便与传统测量指标进行比较,仍然是一个难以解决的挑战。我们展示了一种通过选择性积分测量的FORC分布来重建相分辨磁滞回线的技术。从这些小回线中,可以确定包括矫顽力和饱和场、剩余磁化强度和饱和磁化强度在内的传统指标。为了进行这种分析,必须特别注意对所谓可逆特征的准确量化管理。该技术在三种代表性材料体系上进行了演示,即高各向异性FeCuPt薄膜、Fe纳米点和SmCo/Fe交换弹簧磁体薄膜,并且与直接测量的主回线以及相分离回线显示出极好的一致性。