基于稀土的金属有机骨架作为催化转化的多功能平台。
Rare-Earth-Based Metal-Organic Frameworks as Multifunctional Platforms for Catalytic Conversion.
机构信息
Tianjin Key Lab for Rare Earth Materials and Applications, Center for Rare Earth and Inorganic Functional Materials, School of Materials Science and Engineering & National Institute for Advanced Materials, Nankai University, Tianjin, 300350, P. R. China.
School of Chemistry and Chemical Engineering, Inner Mongolia Key Lab of Nanoscience and Nanotechnology, Inner Mongolia Engineering and Technology Research Center for Catalytic Conversion and Utilization of Carbon Resource Molecules, Inner Mongolia University, Hohhot, 010021, P. R. China.
出版信息
Small. 2021 Jun;17(22):e2005371. doi: 10.1002/smll.202005371. Epub 2021 Feb 19.
The development of catalytic conversion is very important for human society. In the catalytic process, metal-organic frameworks (MOFs) can be utilized to obtain effective catalysts for their porous structures and adjustable properties. In addition, the introduction of rare-earth (RE) elements with unique properties for catalysts can realize good catalytic performances. Thus, the RE-MOF related catalysts for catalytic conversion are summarized. Due to the cooperation of RE elements and porous MOF structures, the RE-based MOFs can be used as promising catalysts or precursors/supports for other catalysts in the areas of energy conversion, environmental governance, and organic synthesis. These aggregated studies highlight the RE-MOFs as promising candidates for catalytic conversion.
催化转化的发展对人类社会至关重要。在催化过程中，可以利用金属-有机骨架（MOFs）来获得有效的催化剂，因为它们具有多孔结构和可调节的性质。此外，引入具有独特催化性能的稀土（RE）元素可以实现良好的催化性能。因此，对用于催化转化的 RE-MOF 相关催化剂进行了总结。由于 RE 元素和多孔 MOF 结构的协同作用，基于 RE 的 MOFs 可用作能源转化、环境治理和有机合成等领域中其他催化剂的有前途的催化剂或前体/载体。这些综合研究强调了 RE-MOF 作为催化转化的有前途的候选物。
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