College of Environmental Science and Engineering, State Key Laboratory of Pollution Control and Resource Reuse, Ministry of Education Key Laboratory of Yangtze River Water Environment, Tongji University, Shanghai 200092, People's Republic of China.
Key Laboratory of Organic Compound Pollution Control Engineering (MOE), School of Environmental and chemical engineering, Shanghai University, Shanghai 200092, People's Republic of China.
Sci Total Environ. 2021 Aug 15;782:146669. doi: 10.1016/j.scitotenv.2021.146669. Epub 2021 Mar 23.
Nitrogen pollution in water bodies is a serious environmental issue which is commonly treated by various methods such as heterotrophic denitrification. In particular, solid carbon source (SCS)-based denitrification has attracted widespread research interest due to its gradual carbon release, ease of management, and long-term operation. This paper reviews the types and properties of SCSs for different target water bodies. While both natural (wheat straw, wood chips, and fruit shells) and synthetic (polybutylene succinate, polycaprolactone, polylactic acid, and polyhydroxyalkanoates) SCSs are commonly used, it is observed that the denitrification performance of the synthetic sources is generally superior. SCSs have been used in the treatment of wastewater (including aquaculture wastewater), agricultural subsurface drainage, surface water, and groundwater; however, the key research aspects related to SCSs differ markedly based on the target waterbody. These key research aspects include nitrogen pollutant removal rate and byproduct accumulation (ordinary wastewater); water quality parameters and aquatic product yield (recirculating aquaculture systems); temperature and hydraulic retention time (agricultural subsurface drainage); the influence of dissolved oxygen (surface waters); and nitrate-nitrogen load, HRT, and carbon source dosage on denitrification rate (groundwater). It is concluded that SCS-based denitrification is a promising technique for the effective elimination of nitrate-nitrogen pollution in water bodies.
水体中的氮污染是一个严重的环境问题,通常可以通过各种方法进行处理,例如异养反硝化。特别是基于固体碳源(SCS)的反硝化技术由于其逐渐释放碳、易于管理和长期运行而受到广泛关注。本文综述了不同目标水体中 SCS 的类型和特性。虽然天然(麦秸、木屑和果壳)和合成(聚丁二酸丁二醇酯、聚己内酯、聚乳酸和聚羟基烷酸酯)SCS 都被广泛使用,但合成来源的反硝化性能通常更优。SCS 已被用于处理废水(包括养殖废水)、农业地下水排水、地表水和地下水;然而,基于目标水体,SCS 的关键研究方面存在显著差异。这些关键研究方面包括氮污染物去除率和副产物积累(普通废水);水质参数和水产养殖产量(循环水产养殖系统);温度和水力停留时间(农业地下水排水);溶解氧的影响(地表水);以及硝酸盐氮负荷、HRT 和碳源剂量对反硝化速率的影响(地下水)。结论是,基于 SCS 的反硝化技术是有效消除水体中硝酸盐氮污染的一种很有前途的技术。