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用于柔性纸质光电探测器的二硫化钼/硒化钨纳米杂化物

MoS/WSenanohybrids for flexible paper-based photodetectors.

作者信息

Pataniya Pratik M, Patel Vikas, Sumesh C K

机构信息

Department of Physical Science, P. D. Patel Institute of Applied Sciences, Charotar University of Science and Technology, CHRUSAT, Changa-388421, Gujarat, India.

Sophisticated Instrumentation Centre for Applied Research and Testing (SICART), Vallabh Vidyanagar, Anand, Gujarat-388 120, India.

出版信息

Nanotechnology. 2021 May 12;32(31). doi: 10.1088/1361-6528/abf77a.

Abstract

Flexible photodetectors functionalized by transition metal dichalcogenides have attracted great attention due to their excellent photo-harvesting efficiency. However, the field of optoelectronics still requires advancement in the production of large-area, broad band and flexible photodetectors. Here we report a flexible, stable, broad band and fast photodetector based on a MoS/WSeheterostructure on ordinary photocopy paper with pencil-drawn graphite electrodes. Ultrathin MoS/WSenanohybrids have been synthesized by an ultrahigh yield liquid-phase exfoliation technique. The thin sheets of WSe, and MoScontain two to four layers with a highly c-oriented crystalline structure. Subsequently, the photodetector was exploited under ultra-broad spectral range from 400 to 780 nm. The photodetector exhibits excellent figure of merit such as on/off ratio of the order of 10, photoresponsivity of 124 mA Wand external quantum efficiency of 23.1%. Encouragingly, rise/decay time of about 0.1/0.3 s was realized, which is better than in previous reports on paper-based devices.

摘要

由过渡金属二硫属化物功能化的柔性光电探测器因其优异的光捕获效率而备受关注。然而,光电子学领域在大面积、宽带和柔性光电探测器的生产方面仍需要取得进展。在此,我们报道了一种基于普通复印纸上带有铅笔绘制石墨电极的MoS₂/WSe₂异质结构的柔性、稳定、宽带且快速的光电探测器。通过超高产率液相剥离技术合成了超薄MoS₂/WS₂纳米杂化物。WSe₂和MoS₂的薄片包含两到四层,具有高度c取向的晶体结构。随后,该光电探测器在400至780 nm的超宽光谱范围内进行了测试。该光电探测器表现出优异的品质因数,如开/关比约为10³、光响应度为124 mA/W以及外量子效率为23.1%。令人鼓舞的是,实现了约0.1/0.3 s的上升/衰减时间,这比之前关于纸质器件的报道要好。

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