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越南南部一个大都市地区街道灰尘中重金属的污染、来源归因和潜在健康风险。

Contamination, source attribution, and potential health risks of heavy metals in street dust of a metropolitan area in Southern Vietnam.

机构信息

Faculty of Chemical & Food Technology, Ho Chi Minh City University of Technology and Education, Thu Duc, Ho Chi Minh City, 700000, Vietnam.

Department of Environmental Sciences, Saigon University, Ho Chi Minh City, 700000, Vietnam.

出版信息

Environ Sci Pollut Res Int. 2021 Sep;28(36):50405-50419. doi: 10.1007/s11356-021-14246-1. Epub 2021 May 6.

Abstract

This study investigates distribution, pollution indices, and potential risk assessment for human health and ecology of eight heavy metals in twenty-five street dust samples collected from metropolitan area-Ho Chi Minh City, Vietnam. Results showed that Zn was of the highest concentration (466.4 ± 236.5 mg/kg), followed by Mn (393.9 ± 93.2 mg/kg), Cu (153.7 ± 64.7 mg/kg), Cr (102.4 ± 50.5 mg/kg), Pb (49.6 ± 21.4 mg/kg), Ni (36.2 ± 15.4 mg/kg), Co (7.9 ± 1.9 mg/kg), and Cd (0.5 ± 0.5 mg/kg). The principal component analysis revealed that three sources of heavy metals measured in street dust include vehicular activities (32.38%), mixed source of vehicular and residential activities (26.72%), and mixture of industrial and natural sources (20.23%). The geo-accumulation index values showed levels of non-pollution to moderately pollution for Mn and Co; moderately pollution for Ni; moderately to strongly pollution for Cd, Cr, and Pb; and strongly pollution for Cu and Zn. The potential ecological risk values of all sampling sites were close to the high-risk category. Zn (28.9%), Cu (25.4%), and Mn (24.4%) dominantly contributed to the ecological risk. For non-carcinogenic risk, the hazard quotient values for both children and adults were within a safety level. For carcinogenic risk, the TCR was about 3 times higher than TCR, but still within a tolerable limit (1 × 10 to 1 × 10) of cancer risk. Cr was a major contribution to potential risks in humans. Such studies on heavy metal in street dust are crucial but are still limited in Vietnam/or metropolitan area in Southeast Asia. Therefore, this study can fill the information gap about heavy metal contaminated street dust in a metropolitan area of Vietnam.

摘要

本研究调查了来自越南胡志明市大都市地区的 25 个街道灰尘样本中八种重金属的分布、污染指数和对人类健康和生态的潜在风险评估。结果表明,锌的浓度最高(466.4 ± 236.5 mg/kg),其次是锰(393.9 ± 93.2 mg/kg)、铜(153.7 ± 64.7 mg/kg)、铬(102.4 ± 50.5 mg/kg)、铅(49.6 ± 21.4 mg/kg)、镍(36.2 ± 15.4 mg/kg)、钴(7.9 ± 1.9 mg/kg)和镉(0.5 ± 0.5 mg/kg)。主成分分析表明,街道灰尘中测量的重金属有三个来源,包括车辆活动(32.38%)、车辆和住宅活动混合源(26.72%)和工业和自然源混合物(20.23%)。地质累积指数值表明,Mn 和 Co 处于无污染到中度污染水平;Ni 处于中度到强污染水平;Cd、Cr 和 Pb 处于强污染水平;Cu 和 Zn 处于强污染水平。所有采样点的潜在生态风险值都接近高风险类别。Zn(28.9%)、Cu(25.4%)和 Mn(24.4%)对生态风险的贡献最大。对于非致癌风险,儿童和成人的危害商值都在安全水平内。对于致癌风险,TCR 约是 TCR 的 3 倍,但仍在可接受范围内(1×10 到 1×10)。Cr 是对人类潜在风险的主要贡献者。在越南/东南亚大都市地区,此类街道灰尘重金属研究至关重要,但仍十分有限。因此,本研究可以填补越南大都市地区街道灰尘重金属污染信息的空白。

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