Hassanpour E, Weber M C, Zemp Y, Kuerten L, Bortis A, Tokunaga Y, Taguchi Y, Tokura Y, Cano A, Lottermoser Th, Fiebig M
Department of Materials, ETH Zurich, Zurich, Switzerland.
Department of Physics, ETH Zurich, Zurich, Switzerland.
Nat Commun. 2021 May 12;12(1):2755. doi: 10.1038/s41467-021-22808-7.
Systems with long-range order like ferromagnetism or ferroelectricity exhibit uniform, yet differently oriented three-dimensional regions called domains that are separated by two-dimensional topological defects termed domain walls. A change of the ordered state across a domain wall can lead to local non-bulk physical properties such as enhanced conductance or the promotion of unusual phases. Although highly desirable, controlled transfer of these properties between the bulk and the spatially confined walls is usually not possible. Here, we demonstrate this crossover by confining multiferroic DyTbFeO domains into multiferroic domain walls at an identified location within a non-multiferroic environment. This process is fully reversible; an applied magnetic or electric field controls the transformation. Aside from expanding the concept of multiferroic order, such interconversion can be key to addressing antiferromagnetic domain structures and topological singularities.
具有铁磁性或铁电性等长程有序的系统表现出均匀但取向不同的三维区域,称为畴,这些畴由二维拓扑缺陷即畴壁分隔开。畴壁两侧有序状态的变化会导致局部非体相物理性质,如增强的电导率或促进异常相的形成。尽管这非常令人期待,但通常无法实现这些性质在体相和空间受限的畴壁之间的可控转移。在此,我们通过在非多铁性环境中的特定位置将多铁性DyTbFeO畴限制为多铁性畴壁来展示这种转变。这个过程是完全可逆的;施加的磁场或电场控制着这种转变。除了扩展多铁性有序的概念之外,这种相互转换对于解决反铁磁畴结构和拓扑奇点可能至关重要。