You Ziyi, Liao Yulong, Li Xin, Fan Jiajie, Xiang Quanjun
State Key Laboratory of Electronic Thin Film and Integrated Devices, School of Electronic Science and Engineering, University of Electronic Science and Technology of China, Chengdu 610054, P. R. China.
Nanoscale. 2021 Jun 3;13(21):9463-9504. doi: 10.1039/d1nr02224e.
Recently, the emerging two-dimensional material MXene enjoys a high reputation due to its fascinating characteristics and shines in various research fields. Among them, MXene has received increasing attention and favor from the photocatalysis community due to its regular planar structure, outstanding metal conductivity, surface adjustable chemical properties, abundant derivatives, and excellent optical and thermal properties. There is no doubt that the introduction of MXene has endowed the photocatalytic system with extraordinary performance and has made an important impact in the field of advanced catalysis and chemical technology. Herein, on the one hand, we summarize the synthetic route of MXenes and MXene-derived 0D quantum dots (MQDs), and propose the corresponding improved synthetic strategies for the defects of MXenes obtained by the current synthetic methods. On the other hand, recent progress in MXene-based photocatalysts has been reviewed to provide a comprehensive dissection of their designs and applications. It is highly anticipated that these will present researchers with a one-stop point for the state-of-the-art development of MXene-based photocatalysts. Finally, the future opportunities and challenges of MXenes in the flourishing field of photocatalysis are also discussed.
近年来,新兴的二维材料MXene因其迷人的特性而享有盛誉,并在各个研究领域大放异彩。其中,MXene因其规则的平面结构、出色的金属导电性、可调节的表面化学性质、丰富的衍生物以及优异的光学和热学性质,受到了光催化领域越来越多的关注和青睐。毫无疑问,MXene的引入赋予了光催化体系非凡的性能,并在先进催化和化学技术领域产生了重要影响。在此,一方面,我们总结了MXenes和MXene衍生的零维量子点(MQDs)的合成路线,并针对当前合成方法获得的MXenes的缺陷提出了相应的改进合成策略。另一方面,综述了基于MXene的光催化剂的最新进展,以全面剖析其设计和应用。高度期望这些内容能为研究人员提供基于MXene的光催化剂最新发展的一站式参考。最后,还讨论了MXenes在蓬勃发展的光催化领域的未来机遇和挑战。