May A, Saccone M, van den Berg A, Askey J, Hunt M, Ladak S
School of Physics and Astronomy, Cardiff University, Cardiff, UK.
Center for Nonlinear Studies, Los Alamos National Laboratory, Los Alamos, NM, USA.
Nat Commun. 2021 May 28;12(1):3217. doi: 10.1038/s41467-021-23480-7.
Magnetic charge propagation in spin-ice materials has yielded a paradigm-shift in science, allowing the symmetry between electricity and magnetism to be studied. Recent work is now suggesting the spin-ice surface may be important in mediating the ordering and associated phase space in such materials. Here, we detail a 3D artificial spin-ice, which captures the exact geometry of bulk systems, allowing magnetic charge dynamics to be directly visualized upon the surface. Using magnetic force microscopy, we observe vastly different magnetic charge dynamics along two principal directions. For a field applied along the surface termination, local energetics force magnetic charges to nucleate over a larger characteristic distance, reducing their magnetic Coulomb interaction and producing uncorrelated monopoles. In contrast, applying a field transverse to the surface termination yields highly correlated monopole-antimonopole pairs. Detailed simulations suggest it is the difference in effective chemical potential as well as the energy landscape experienced during dynamics that yields the striking differences in monopole transport.
自旋冰材料中的磁荷传播在科学领域引发了范式转变,使得电与磁之间的对称性得以研究。近期的研究表明,自旋冰表面在介导此类材料中的有序化及相关相空间方面可能具有重要作用。在此,我们详细介绍一种三维人工自旋冰,它捕捉了块体系统的精确几何结构,使得磁荷动力学能够在表面直接可视化。利用磁力显微镜,我们观察到沿两个主方向的磁荷动力学存在巨大差异。对于沿表面终止方向施加的磁场,局部能量迫使磁荷在更大的特征距离上成核,降低它们的磁库仑相互作用并产生不相关的单极子。相比之下,垂直于表面终止方向施加磁场会产生高度相关的单极 - 反单极子对。详细的模拟表明,有效化学势的差异以及动力学过程中所经历的能量景观导致了单极子输运的显著差异。