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有机/无机杂化纤维：用于电化学能源应用的可控结构

Organic/Inorganic Hybrid Fibers: Controllable Architectures for Electrochemical Energy Applications.

作者信息

Zhang Fangzhou, Sherrell Peter C, Luo Wei, Chen Jun, Li Wei, Yang Jianping, Zhu Meifang

机构信息

State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, P. R. China.

Department of Chemical Engineering, The University of Melbourne, Parkville, VIC, 3010, Australia.

出版信息

Adv Sci (Weinh). 2021 Nov;8(22):e2102859. doi: 10.1002/advs.202102859. Epub 2021 Oct 11.

DOI:10.1002/advs.202102859
PMID:34633752
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC8596128/
Abstract

Organic/inorganic hybrid fibers (OIHFs) are intriguing materials, possessing an intrinsic high specific surface area and flexibility coupled to unique anisotropic properties, diverse chemical compositions, and controllable hybrid architectures. During the last decade, advanced OIHFs with exceptional properties for electrochemical energy applications, including possessing interconnected networks, abundant active sites, and short ion diffusion length have emerged. Here, a comprehensive overview of the controllable architectures and electrochemical energy applications of OIHFs is presented. After a brief introduction, the controllable construction of OIHFs is described in detail through precise tailoring of the overall, interior, and interface structures. Additionally, several important electrochemical energy applications including rechargeable batteries (lithium-ion batteries, sodium-ion batteries, and lithium-sulfur batteries), supercapacitors (sandwich-shaped supercapacitors and fiber-shaped supercapacitors), and electrocatalysts (oxygen reduction reaction, oxygen evolution reaction, and hydrogen evolution reaction) are presented. The current state of the field and challenges are discussed, and a vision of the future directions to exploit OIHFs for electrochemical energy devices is provided.

摘要

有机/无机杂化纤维（OIHFs）是一种引人关注的材料，具有固有的高比表面积和柔韧性，同时具备独特的各向异性特性、多样的化学成分以及可控的杂化结构。在过去十年中，出现了具有卓越性能的先进OIHFs，可用于电化学能源应用，包括拥有相互连接的网络、丰富的活性位点以及短的离子扩散长度。在此，本文对OIHFs的可控结构及其在电化学能源方面的应用进行了全面概述。在简要介绍之后，通过对整体、内部和界面结构的精确剪裁，详细描述了OIHFs的可控构建。此外，还介绍了几种重要的电化学能源应用，包括可充电电池（锂离子电池、钠离子电池和锂硫电池）、超级电容器（三明治状超级电容器和纤维状超级电容器）以及电催化剂（氧还原反应、析氧反应和析氢反应）。讨论了该领域的现状和挑战，并展望了利用OIHFs开发电化学能源装置的未来方向。

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